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| 1 | A review of the synthesis and application of zeolites from coal-based solid wastes显示文摘Zeolite derived from coal-based solid wastes(coal gangue and coal fly ash)can overcome the environmental problems caused by coal-based solid wastes and achieve valuable utilization.In this paper,the physicochemical properties of coal gangue and coal fly ash are introduced.The mechanism and application characteristics of the pretreatment processes for zeolite synthesis from coal-based solid wastes are also introduced.The synthesis processes of coal-based solid waste zeolite and their advantages and disadvantages are summarized.Furthermore,the application characteristics of various coal-based solid waste zeolites and their common application fields are illustrated.Finally,we propose an alkaline fusion-assisted supercritical hydrothermal crystallization as an efficient method for synthesizing coal-based solid waste zeolites.In addition,more attention should be given to the recycling of alkaline waste liquid and the application of coal-based solid waste zeolites in the field of volatile organic compound adsorption removal. | Xiaoyu Zhang Chunquan Li Shuilin Zheng Yonghao Di Zhiming Sun | 2022 | International Journal of Minerals,Metallurgy and Materials2022，29，1： | 10 |
| 2 | Hierarchical assembly of highly efficient visible-light-driven Ag/g-C_(3)N_(4)/kaolinite composite photocatalyst for the degradation of ibuprofen显示文摘A novel Ag/g-C_(3)N_(4)/kaolinite composite photocatalyst was fabricated for the first time through a two-step assembly strategy by employing in situ calcination and a photodeposition process.The synthesized Ag/g-C_(3)N_(4)/kaolinite composite reached a higher degradation rate of ibuprofen(IBP)with a reaction rate constant of 0.0113 min^(-1) at an Ag content of 7% under visible-light irradiation,which was approximately 1.87 times that of the Ag/g-C_(3)N_(4) composite.Based on the physicochemical properties,the enhanced photocatalytic activity was attributed to the stronger adsorption property,wider photoresponse range and more efficient separation and transfer of electron-hole pairs.Furthermore,the incorporation of monodispersed Ag nanoparticles onto the g-C_(3)N_(4)/kaolinite sheets provided more reactive sites for the IBP degradation.In addition,according to the EPR study and trapping experiments,it was demonstrated that holes(h^(+))should be the key reactive species.A possible pathway of IBP degradation was also proposed based on the detected intermediates.Overall,the results of this work may facilitate the design of a novel visible-light-driven photocatalyst with a high efficiency that is derived from a natural mineral for environmental remediation. | Zhiming Sun Xiangwei Zhang Xiongbo Dong Xiaorui Liu Ye Tan Fang Yuan Shuilin Zheng Chunquan Li | 2020 | Journal of Materiomics2020，6，3： | 8 |
| 3 | Thermodynamic Modeling of Fluid-Bearing Natural Gas Inclusions for Geothermometer and Geobarometer of Overpressured Environments in Qiongdongnan Basin, South China Sea显示文摘It is a very difficult problem to directly determine fluid pressure during hydrocarbon migration and accumulation in sedimentary basins. pVt modeling of coupling hydrocarbon fluid inclusion of its coeval aqueous fluid inclusion provides a powerful tool for establishing the relationship of formation pressure evolution with time. Homogenization temperature of fluid inclusion can routinely be measured under microthermometric microscopy. Crushing technique has been employed to obtain the composition of fluid inclusions, and the commercial software VTFLINC easily and rapidly completes the construction of p t phase diagram. The minimum trapping pressure of hydrocarbon fluid inclusion would be then determined in the p t space. In this paper, three samples of YC21 1 1 and YC21 1 4 wells at YC21 1 structural closure, Qiongdongnan basin, South China Sea, were selected for the pVt modeling practice, and the formation pressure coefficient (equals to fluid pressure/hydrostatic pressure) changing trend with time has primarily been established. The modeling results also indicate that the reservoirs of Lingshui and Yacheng formations in YC21 1 structure are within a very high potential system and would have undergone a discharging of thermal fluids through top seal rupture, which depicts that there is a very high risk for natural gas exploration in this area. | Chen Honghan Yao Shuzhen Wang Jiahao Li Chunquan Institute of Resources, China University of Geosciences, Wuhan 430074 | 2002 | Journal of China University of Geosciences2002，13，3： | 7 |
| 4 | Diatomite supported nano zero valent iron with 3D network for peroxymonosulfate activation in efficient degradation of bisphenol A显示文摘Diatomite supported nano zero valent iron(n ZVI)catalyst(NDA)with complex network structure was prepared via a mild reduction precipitation method in this work.The pore structure and pore distribution of NDA can be regulated and controlled through adjusting the loading amount of n ZVI.In general,the nano three-dimensional network formed by n ZVI and diatomite channels greatly increase the specific surface area and pore volume of NDA,and further formed more active sites,which made NDA have better performance in activating PMS to degrade BPA than pure n ZVI.The pseudo-first-order reaction rate constant of 50-NDA(50%-n ZVI/diatomite)is almost 3 times higher than that of pure n ZVI.Besides,the electron paramagnetic resonance(EPR)and radical quenching experiments showed that the activation process was dominated by the sulfate radical(SO_(4)^(-))and hydroxyl radical(·OH)produced by Fe;oxidation.The generated electrons promote the self-decomposition of PMS to produce singlet oxygen(^(1)O_(2)),and then the valence state of iron changes to produce free radicals.In addition,the possible degradation pathway of BPA was inferred from the intermediate products identified by liquid chromatograph-mass spectrometer(LC-MS).This study provides a novel strategy for the design and preparation of three-dimensional composite catalysts derived from natural mineral. | Ye Tan Shuilin Zheng Yonghao Di Chunquan Li Runze Bian Zhiming Sun | 2021 | Journal of Materials Science & Technology2021，，36： | 4 |
| 5 | Effect of Zhu-yuan decoction in patients with chronic rhinosinusitis after functional endoscopic sinus surgery显示文摘OBJECTIVE: To investigate the effectiveness and safety of Zhu-yuan decoction(ZYD) in patients after functional endoscopic sinus surgery(FESS).METHODS: A total of 85 patients were randomized into two groups: 44 were treated with intranasal corticosteroids(INC), and 41 were given Chinese herbal medicine(CHM). Patients with chronic rhinosinusitis(CRS) who underwent FESS were prospectively enrolled in the study. Before surgery, they were evaluated by visual analog scale(VAS), nasal endoscopy, computed tomography(CT), and routine blood test. After surgery, they were randomized to take ZYD or INC for 12 weeks and revaluated by VAS; nasal endoscopy at 4, 8, and 12 weeks;and CT at 12 weeks after surgery.RESULTS: In the both groups, VAS and endoscopyscores decreased significantly at 4, 8, and 12 weeks,and CT scores after treatment declined at 12 weeks compared with baseline scores. No significant differences were observed with regard to postoperative VAS, endoscopy, or CT scores between groups.ZYD, combined with surgery, can reduce VAS, nasal endoscopy, and CT scores and has the same efficacy and safety profile as INC in post-FESS management.No fatalities or major adverse events occurred in either group.CONCLUSION: Our findings suggest that ZYD has similar effects and safety profiles in patients after FESS compared with INC. | Li Jing Zheng Chunquan Lin Hai Yang Chen Gu Siyuan Wang Yi Duan Honggang | 2018 | Journal of Traditional Chinese Medicine2018，38，1： | 3 |
| 6 | Engineered tunneling layer with enhaneed impact ionization for detection improvement in graphene/silicon heterojunction photodetectors显示文摘Here,an engineered tunneling layer enhanced photocurrent multiplication through the impact ionization effect was proposed and experimentally demonstrated on the graphene/silic on heterojunction photodetectors.With con sidering the suitable band structure of the insulation material and their special defect states,an atomic layer deposition(ALD)prepared wide-bandgap insulating(WBI)layer of AIN was introduced into the interface of graphene/silicon heterojunction.The promoted tunneling process from this designed structure dem on strated that can effectively help the impact ionization with photogain not only for the regular minority carriers from silicon,but also for the novel hot carries from graphene.As a result,significantly enhanced photocurrent as well as simultaneously decreased dark current about one order were accomplished in this graphene/insulation/silicon(GIS)heterojunction devices with the optimized AIN thickness of〜15 nm compared to the conventional graphene/silicon(GS)devices.Specifically,at the reverse bias of-10 V,a 3.96-A W_1 responsivity with the photogain of~5.8 for the peak response under 850-nm light illumination,and a 1.03-A W_1 responsivity with~3.5 photogain under the 365 nm ultraviolet(UV)illumination were realized,which are even remarkably higher than those in GIS devices with either AI2O3 or the commonly employed SiO2 insulation layers.This work dem on strates a universal strategy to fabricate broad ba nd,low-cost and high-performance photo-detecting devices towards the graphene-silicon optoelectronic integration. | Jun Yin Lian Liu Yashu Zang Anni Ying Wenjie Hui Shusen Jiang Chunquan Zhang Tzuyi Yang Yu-Lun Chueh Jing Li Junyong Kang | 2021 | Light(Science & Applications)2021，10，6： | 3 |
| 7 | Targeting a novel inducible GPX4 alternative isoform to alleviate ferroptosis and treat metabolic-associated fatty liver disease显示文摘Metabolic-associated fatty liver disease(MAFLD),which is previously known as non-alcoholic fatty liver disease(NAFLD),represents a major health concern worldwide with limited therapy.Here,we provide evidence that ferroptosis,a novel form of regulated cell death characterized by iron-driven lipid peroxidation,was comprehensively activated in liver tissues from MAFLD patients.The canonical-GPX4(cGPX4),which is the most important negative controller of ferroptosis,is downregulated at protein but not mRNA level.Interestingly,a non-canonical GPX4 transcript-variant is induced(inducible-GPX4,iGPX4)in MAFLD condition.The high fat-fructose/sucrose diet(HFFD)and methionine/choline-deficient diet(MCD)-induced MAFLD pathologies,including hepatocellular ballooning,steatohepatitis andfibrosis,were attenuated and aggravated,respectively,in cGPX4-and iGPX4-knockin mice.cGPX4 and iGPX4 isoforms also displayed opposing effects on oxidative stress and ferroptosis in hepatocytes.Knockdown of iGPX4 by siRNA alleviated lipid stress,ferroptosis and cell injury.Mechanistically,the triggered iGPX4 interacts with cGPX4 to facilitate the transformation of cGPX4 from enzymatic-active monomer to enzymatic-inactive oligomers upon lipid stress,and thus promotes ferroptosis.Co-immunoprecipitation and nano LC–MS/MS analyses confirmed the interaction between iGPX4 and cGPX4.Our results reveal a detrimental role of non-canonical GPX4 isoform in ferroptosis,and indicate selectively targeting iGPX4 may be a promising therapeutic strategy for MAFLD. | Jie Tong Dongjie Li Hongbo Meng Diyang Sun Xiuting Lan Min Ni Jiawei Ma Feiyan Zeng Sijia Sun Jiangtao Fu Guoqiang Li Qingxin Ji Guoyan Zhang Qirui Shen Yuanyuan Wang Jiahui Zhu Yi Zhao Xujie Wang Yi Liu Shenxi Ouyang Chunquan Sheng Fuming Shen Pei Wang | 2022 | Acta Pharmaceutica Sinica B2022，12，9： | 3 |
| 8 | Enhanced visible-light-assisted peroxymonosulfate activation over MnFe_(2)O_(4) modified g-C_(3)N_(4)/diatomite composite for bisphenol A degradation显示文摘The MnFe_(2) O_(4)/g-C_(3) N_(4)/diatomite composites(Mn/G/D) were prepared via a facile precipitation-calcination method in this study.The Mn/G/D possessed higher specific surface area,lower electron-hole pairs' recombination rate,as well as wider and stronger visible light absorption capacity.Since the synergistic effect between g-C_(3 )N_(4) and MnFe_(2) O_(4),the photogene rated electron could transfer from g-C3 N4 to MnFe_(2) O_(4),which could promote the migration of electrons as well as enhance the photocatalytic activity and peroxymonosulfate(PMS) activation efficiency.Mn/G/D-5% composite displayed the excellent degradation performance of bisphenol A(BPA) with the removal efficiency of 99.9% under PMS/Vis system,which was approximately 2.47 and 63.8 times as high as that of the Mn/G/D-5%/PMS and Mn/G/D-5%/Vis system,respectively.Moreover,negative electricity derived from diatomite surface also promoted the photogenerated carriers' migration,and the degradation rate constant was around 2.4 times higher than that of MnFe_(2) O_(4)/g-C_(3) N_(4)(Mn/G).In addition,quenching experiments showed that both radical pathway(h^(+),·OH,·O_(2)^(-)and SO_(4)·^(-)) and non-radical pathway(^(1) O_(2)) were responsible for the degradation of BPA. | Xiangwei Zhang Chunquan Li Ting Chen Ye Tan Xiaorui Liu Fang Yuan Shuilin Zheng Zhiming Sun | 2021 | International Journal of Mining Science and Technology2021，31，6： | 2 |
| 9 | Robustness of fuzzy reasoning via logically equiva- lence measure显示文摘 | Jin Jianhua Li Yongmin Li Chunquan | 2007 | Information Sciences2007，177，： | 1 |
| 10 | Discovery of novel KRAS-PDEδ inhibitors with potent activity in patient-derived human pancreatic tumor xenograft models显示文摘KRAS-PDEδ interaction is revealed as a promising target for suppressing the function of mutant KRAS. The bottleneck in clinical development of PDEδ inhibitors is the poor antitumor activity of known chemotypes. Here, we identified novel spiro-cyclic PDEδ inhibitors with potent antitumor activity both in vitro and in vivo. In particular, compound 36 l(KD= 127 ± 16 nmol/L) effectively bound to PDEδ and interfered with KRAS-PDEδ interaction. It influenced the distribution of KRAS in Mia PaCa-2 cells, downregulated the phosphorylation of t-ERK and t-AKT and promoted apoptosis of the cells. The novel inhibitor 36 l exhibited significant in vivo antitumor potency in pancreatic cancer patient-derived xenograft(PDX) models. It represents a promising lead compound for investigating the druggability of KRAS-PDEδ interaction. | Long Chen Jing Zhang Xinjing Wang Yu Li Lu Zhou Xiongxiong Lu Guoqiang Dong Chunquan Sheng | 2022 | Acta Pharmaceutica Sinica B2022，12，1： | 1 |
| 11 | Optimized microwave-assisted extraction of total phenolics (TP) from Ipomoea batatas leaves and its antioxidant activity显示文摘 | Jiangfeng Song Dajing Li Chunquan Liu Ying Zhang | 2011 | Innovative Food Science and Emerging Technologies2011，，3： | 1 |
| 12 | Partial purification and characterization of polyphenol oxidase and peroxidase from chestnut kernel显示文摘 | Gong Zhiqing Li Dajing Liu Chunquan | 2015 | LWT-Food Science and Technology2015，60，2： | 1 |
| 13 | A modified simple particle swarm optimization algorithm显示文摘 | Li Chunquan Liu Xiaoping Xu Shaoping | 2012 | Journal of Computational Information Systems2012，8，19： | 1 |
| 14 | Re- search of cloud manufacturing and resource encapsulation technology显示文摘 | LI Chunquan HU Chunyang WANG Yanwei | 2011 | Applied Mechanics and Materials2011，5860，： | 1 |
| 15 | Sugar beet M14 glyoxalase I gene can enhance plant tolerance to abiotic stresses显示文摘 | Chuan Wu Chunquan Ma Yu Pan Shilong Gong Chenxi Zhao Sixue Chen Haiying Li | 2013 | Journal of Plant Research2013，，3： | 1 |
| 16 | Molecularcloning and characterization of a rat sarcoma-like proteinfrom brain (Rab) gene in sugar beet monosomic addi-tional line Ml4 显示文摘 | Li Haiying Ji Lin Ma Chunquan | 2013 | Australin Journal of Crop Sci-ence2013，7，3： | 1 |
| 17 | Salt stress response of membrane proteome of sugar beet monosomic addition line M14显示文摘 | Haiying Li Yu Pan Yongxue Zhang Chuan Wu Chunquan Ma Bing Yu Ning Zhu Jin Koh Sixue Chen | 2015 | Journal of Proteomics2015，，： | 1 |
| 18 | Single-atomic Pt sites anchored on defective Ti0_(2) nanosheets as a superior photocatalyst for hydrogen evolution显示文摘Single-atomic site catalysts have drawn considerable attention because of their maximum atom-utilization efficiency and excellent catalytic activity.In this work,a highly active single-atomic Pt site photocatalyst was synthesized through employing defective Ti0_(2) nanosheets as solid support for photo-catalytic water splitting.It indicated that the surface oxygen vacancies on defective Ti0_(2) nanosheets could effectively stabilize the single-atomic Pt sites through constructing a three-center Ti-Pt-Ti structure.The Ti-Pt-Ti structure can hold the stability of isolated single-atomic Pt sites and facilitate the separation and transfer of photoinduced charge carriers,thereby greatly improving the photocatalytic H2 evolution.Notably,our synthesized photocatalyst exhibited a remarkably enhanced H2 evolution performance,and the H2 production rate is up to 13460.7μmol h^(-1)·g^(-1),which is up to around 29.0 and 4.7 times higher than those of Ti0_(2) nanosheets and Pt nanoparticles-Ti0_(2).In addition,a plausible enhanced reaction mechanism was also proposed combining with photo-electrochemical characterizations and density functional theoiy(DFT)calculation results.Ultimately,it is believed that this work highlights the benefits of a single-site catalyst and paves the way to rationally design the highly active and stable single-atomic site photocatalysts on metal oxide support. | Xiaolong Hu Junying Song Jingli Luo Hao Zhang Zhiming Sun Chunquan Li Shuilin Zheng Qingxia Liu | 2021 | Journal of Energy Chemistry2021，30，11： | 1 |
| 19 | Molecularcloning and characterization of a rat sarcoma-like pro-tein from brain (Rab) gene in sugar beet monosomicadditional line Ml4 显示文摘 | Haiying Li Lin Ji Chunquan Ma | 2013 | Australin Journal of CropScience2013，7，3： | 1 |
| 20 | Hydrocarbon Inclusion Characteristics in the Cambrian-Ordovician Carbonates of the TS2 Well:Implication for Deep Hydrocarbon Exploration in the Tahe Oilfield,Tarim Basin,Northwest China显示文摘Going deep has been the strategy for the sustainable development of the Tahe Oilfield.Following the TS1 well in block 1,which revealed excellent combinations of hydrocarbon generation,migration and accumulation in the deeper parts of the Tarim Basin,the TS2 well was drilled to learn more about the prospectivity in the deeper parts of the main blocks of the Tahe Oilfield.Seventeen core samples were collected to perform fluid inclusion studies,including petrography,fluorescence microspectrometry,and microthermometry.The results show that the deeper parts of the Tahe Oilfield have a good hydrocarbon potential.The Cambrian source rocks can supply sufficient oil for not only the Cambrian reservoirs,but also for the Lower Ordovician reservoirs.The CambrianOrdovician carbonates reservoirs experienced at least three oil charging events and one late gas charging event.Oil accumulations formed in the early stage of basin evolution were likely destroyed in the late stage with deep burial,tectonic movements,or invasion of hydrothermal fluids.Therefore,the deep hydrocarbon exploration of the Tahe Oilfield,even the whole Tarim Basin,should focus on gas accumulations,although oil accumulations,especially in Cambrian reservoirs,cannot be neglected. | LI Chunquan CHEN Honghan | 2015 | Acta Geologica Sinica(English Edition)2015，89，3： | 1 |
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