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| 1 | Vapor-phase growth of high-quality wafer-scale two-dimensional materials显示文摘Emerging two-dimensional(2D)materials have stimulated tremendous scientific and industrial interests due to their diverse and tunable physical,chemical,and mechanical properties.The scalable production of high-quality wafer-scale 2D materials has become significantly essential to bring us closer to practical industrial applications,particularly in electronic devices.Vapor-phase growth provides attractive opportunities for the synthesis of large-area and high-quality 2D materials.In this review,we will emphasize vapor-phase growth strategies from three aspects,including suppressing nucleation,seamless stitching,and evolutionary selection growth.We discuss the general understanding of the related fundamental mechanism and specific parameter optimization from precursors and substrate design to the adjusting of growth parameters(temperature and pressure).Meanwhile,we present other strategies to produce various kinds of wafer-scale 2D materials.Finally,we conclude the current challenges and future directions in this developing field.This work may inspire researchers to better design routes in the synthesis of wafer-scale 2D materials with high quality. | Xin Tong Keli Liu Mengqi Zeng Lei Fu | 2019 | InfoMat2019，1，4： | 5 |
| 2 | Two-dimensional Metal-Organic Frameworks as Electrocatalysts for Oxygen Evolution Reaction显示文摘Oxygen evolution reaction(OER)plays an important role in many electrochemical systems.However,its sluggish kinetics severely limits the development of next-generation energy technologies.Recently,two-dimensional(2D)metal-organic frameworks(MOFs)have attracted much attention as a class of promising electrocatalysts.Their diverse components and tunable structures provide a new platform to design and explore ideal eleclrocatalysts.The ultrathin characteristics including high specific surface area,abundant exposed metal sites and fast electronic transfer further promote the electrocatalytic performance of 2D MOFs.Therefore,many attempts have been made in svntliesizing 2D MOF-based electrocatalysts in recent years.This review focuses on the strategies to fabricate 2D MOFs with high electrocatalytic performances for OER.The discussion on challenge and development of their electrocatalytic application is also presented. | LEI Jia ZENG Mengqi FU Lei | 2020 | Chemical Research in Chinese Universities2020，36，4： | 2 |
| 3 | SETD8 induces stemness and epithelial–mesenchymal transition of pancreatic cancer cells by regulating ROR1 expression显示文摘Pancreatic cancer(PC)is one of the most deadly diseases,and its incidence is increasing year by year.The methyltransferase SETD8 has been demonstrated to play an important role in tumor cell proliferation and metastasis.However,little is known about whether SETD8 could affect the invasion and metastasis of PC and the mechanism underlying the regulation.Based on our previous report,here,we further found that SETD8 could promote the invasion and migration of PC cells by inducing the expression of receptor tyrosine kinase-like orphan receptor 1(ROR1).ROR1 was predominantly upregulated in PC tissues and was correlated with lymph node metastasis and worse prognosis.Mechanistically,SETD8 mediated ROR1 activity and regulated PC cells invasion and migration,although promoting the expression of stemness and epithelial–mesenchymal transition-related molecules.This promotion effect disappeared when the catalytically inactive mutant SETD8 was overexpressed,which could be counteracted by the SETD8-specific methyltransferase inhibitor UNC0379.Collectively,our results demonstrate that SETD8 may be a novel prognostic factor and a therapeutic target of PC. | Mengqi Liu Yihua Shi Qiangsheng Hu Yi Qin Shunrong Ji Wensheng Liu Qifeng Zhuo Guixiong Fan Zeng Ye Changfeng Song Xianjun Yu Xiaowu Xu Wenyan Xu | 2021 | Acta Biochimica et Biophysica Sinica2021，53，12： | 2 |
| 4 | FGFBPI-mediated crosstalk between fibroblasts and pancreatic cancer cells via FGF22/FGFR2 promotes invasion and metastasis of pancreatic cancer显示文摘Fibroblast growth factor-binding protein 1(FGFBP1)promotes fibroblast growth factor(FGF)activity by releasing FGFs from extracellular matrix storage.We previously reported that the tumor suppressor F-box and WD repeat domain-containing 7 suppresses FGFBP1 by reducing expression of c-Myc,which inhibits the proliferation and migration of pancreatic cancer cells.However,the potential mechanism by which FGFBP1 facilitates pancreatic ductal adenocarcinoma(PDAC)remains unexplored.In this study,we focused on the function of FGFBP1 in the interplay between cancer-associated fibroblasts(CAFs)and pancreatic cancer cells(PCCs).Decreased FGF22 expression was detected in CAFs co-cultured with PCCs with FGFBP1 abrogation,which was verified in the cell culture medium by enzyme-linked immunosorbent assay.Active cytokine FGF22 significantly facilitated the migration and invasion of PANC-1 and Mia PaCa-2 cells.The number of penetrating PCCs cocultured with CAFs with FGF22 abrogation was significantly less than that of the control group.Interestingly,higher expressions of FGF22 and fibroblast growth factor receptor 2(FGFR2)were associated with worse prognosis of patients with PDAC and FGFR2,an independent prognostic marker of PDAC.The PANC-1 and Mia PaCa-2 cells with silenced FGFR2 showed weaker invasion and metastasis,even if these cells were simultaneously treated with cytokine FGF22.These results revealed that FGFBPI-mediated interaction between CAFs and PCCs via FGF22/FGFR2 facilitates the migration and invasion of PCCs.FGFR2 could act as a prognostic marker for patients with PDAC. | Zheng Zhang Yi Qin Shunrong Ji Wenyan Xu Mengqi Liu Qiangsheng Hu Zeng Ye Guixiong Fan Xianjun Yu Wensheng Liu Xiaowu Xu | 2021 | Acta Biochimica et Biophysica Sinica2021，53，8： | 2 |
| 5 | Finding Main Causes of Elevator Accidents via Multi-Dimensional Association Rule in Edge Computing Environment显示文摘In order to discover the main causes of elevator group accidents in edge computing environment, a multi-dimensional data model of elevator accident data is established by using data cube technology, proposing and implementing a method by combining classical Apriori algorithm with the model, digging out frequent items of elevator accident data to explore the main reasons for the occurrence of elevator accidents. In addition, a collaborative edge model of elevator accidents is set to achieve data sharing, making it possible to check the detail of each cause to confirm the causes of elevator accidents. Lastly the association rules are applied to find the law of elevator Accidents. | Hongman Wang Mengqi Zeng Zijie Xiong Fangchun Yang | 2017 | China Communications2017，14，11： | 2 |
| 6 | Space-confined growth of metal halide perovskite crystal films显示文摘Metal halide perovskites,as a new generation of optoelectronic materials,have attracted a great deal of interest due to their remarkable intrinsic properties.Due to the excellent optoelectronic properties,the perovskite crystals are widely used in lasers,photodetectors,X-ray detectors and solar cells.Considering the device performance and fabrication requirements,proper thickness of the crystal is required to avoid carrier loss and simultaneously ensure sufficient light absorption,which can realize the full potential of its excellent carrier transport property.Thus,the fabrication of perovskite crystal in a thin film with an adjustable thickness is highly desirable.The space-confined method has been demonstrated to be an effective way of preparing perovskite with controlled thickness.In this method,the thickness of perovskite can be regulated flexibly in a geometric confined space.Moreover,the size,quality and architecture of perovskite crystal films are also major concerns for practical photoelectric devices,which can also be optimized by the space-confined method owing to its good adaptability towards various modified strategies.In a word,the space-confined method is not only a simple and conventional way to adjust the thickness of perovskite crystal films,but also provides a platform to optimize their size,quality and architecture through applying appropriate strategies to the confined space.Herein,we review the space-confined growth of perovskite crystal films.Particularly,various modified strategies based on the space-confined method applied to the optimization of thickness,size,quality and architecture are highlighted.Then the stability investigating and component regulating of perovskite crystal films would be also mentioned.Furthermore,the correlation between the perovskite thickness and the device performance is discussed.Finally,several key challenges and proposed solutions of perovskite thin films based on the space-confined method are discussed. | Linyi Li Jinxin Liu Mengqi Zeng Lei Fu | 2021 | Nano Research2021，14，6： | 2 |
| 7 | Modification of poly (hutylene terephthalate) with core shell nanoparticles containing UV-absorber显示文摘 | Liu Lei You Bin Zeng Mengqi | 2014 | Journal of Polymer Research2014，21，4： | 1 |
| 8 | A Liquid Metal Reaction System for Advanced Material Manufacturing显示文摘CONSPECTUS:Liquid metal exhibits the unique advantages of both the liquid and metal,including excellent deformability,high thermal conductivity,and electrical conductivity.The exploration of liquid metal is a new opportunity and revolution for the application of metal materials,including the flexible devices,catalysis,microfluidic,and drug delivery.In addition to the above applications,the characteristics of excellent inclusive ability with the majority of the elements and abundant vacancies in the bulk make it a new type of reaction medium different from traditional aqueous and organic solutions,exhibiting great potential in the precise construction of materials.To date,the research of using liquid metal as a reaction system to synthesize materials is still in its infancy.When acting as a reaction system,the vacancies inside and the smooth layering surfaces without grain boundaries allow liquid metals to encapsulate heterogeneous atoms,confine the precursors in atomically thick layers and realize the self-limiting growth of 2D material.Besides,the good rheological property makes it possible to construct 2D arrays on its surface.Except for the properties mentioned above,as a kind of metal,its excellent electrical conductivity and ductility provide a new idea for the preparation of composite materials in the energy field.Indeed,liquid metals provide attractive prospects in manufacturing advanced materials including 2D materials and functional composite materials.Thus,this Account aims to focus on the controllable fabrication of 2D materials and functional composite materials by liquid metals.Based on the characteristics of the surface layering and solidification and of excellent fluidity,the self-limited growth and ordered arrangement of 2D materials on liquid metal surfaces can be achieved,which enriches the material structures and leads to new properties.By constructing an in situ synthesis and observation system,the growth and assembly behavior of 2D materials on the liquid metal can be observed directly.Combining the electrical property,deformability,ductility,and high inclusive ability with other materials,the liquid metal reaction system can also realize the preparation of new functional composite materials toward various applications,such as the energy field.Except for the 2D materials and functional composite materials mentioned here,liquid metals also provide more possibilities for fabricating other promising materials,like wafer-scale semiconductors,magic-angle graphene,flexible functional materials,biomedical materials,and so on.The research concerning the manufacturing of advanced materials on liquid metals is still in its infancy.We believe that the development of related technologies offering in-depth investigation and theoretical understanding on liquid metals will lay a solid foundation for the basic research and practical application of more advanced materials. | Mengqi Zeng Linyang Li Xiaohui Zhu Lei Fu | 2021 | Accounts of Materials Research2021，2，8： | 1 |
| 9 | Carbon-black-filled polyolefine as a positive temperature coefficient material:effect of composition, processing, and filler treatment显示文摘 | Yu Gang Zhang Mengqi Zeng Hong | 1998 | Journal of Applied Polymer Science1998，70，3： | 1 |
| 10 | Recent progress in synthesis and properties of 2D room-temperature ferromagnetic materials显示文摘Two-dimensional(2D)ferromagnetic materials have important applications in optics,spintronics,biomedicine,and energy conversion fields.To achieve higher integration and continue Moore's Law,it is necessary to search for 2D ferromagnetic materials.However,the low Curie temperature(Tc)of most 2D ferromagnetic materials seriously hinders their practical applications.Therefore,the search for room-temperature 2D ferromagnetic materials is of great significance for the advancement of technological applications.This article provides a systematic and comprehensive review of the synthesis methods of room-temperature 2D ferromagnetic materials that have been discovered and created to date,as well as an overview of the physical properties of the 2D ferromagnetic materials.Finally,the challenges and prospects of the room-temperature 2D ferromagnetic materials in the fields of synthesis and application are briefly summarized. | Lixuesong Han Tingting Cheng Yiran Ding Mengqi Zeng Lei Fu | 2023 | Science China Chemistry2023，66，11： | 0 |
| 11 | Arbitrarily polarized bound states in the continuum with twisted photonic crystal slabs显示文摘Arbitrary polarized vortex beam induced by polarization singularity offers a new platform for both classical optics and quantum entanglement applications.Bound states in the continuum(BICs)have been demonstrated to be associated with topological charge and vortex polarization singularities in momentum space.For conventional symmetric photonic crystal slabs(PhCSs),BIC is enclosed by linearly polarized far fields with winding angle of 2π,which is unfavorable for high-capacity and multi-functionality integration-optics applications.Here,we show that by breakingσz-symmetry of the PhCS,asymmetry in upward and downward directions and arbitrarily polarized BIC can be realized with a bilayer-twisted PhCS.It exhibits elliptical polarization states with constant ellipticity angle at every point in momentum space within the vicinity of BIC.The topological nature of BIC reflects on the orientation angle of polarization state,with a topological charge of 1 for any value of ellipticity angle.Full coverage of Poincarésphere(i.e.,-π/4≤X≤4 and-π/2≤ψ≤π/2)and higher-order Poincarésphere can be realized by tailoring the twist angles.Our findings may open up new avenues for applications in structured light,quantum optics,and twistronics for photons. | Haoye Qin Zengping Su Mengqi Liu Yixuan Zeng Man-Chung Tang Mengyao Li Yuzhi Shi Wei Huang Cheng-Wei Qiu Qinghua Song | 2023 | Light(Science & Applications)2023，12，4： | 0 |
| 12 | CATIRI:An Efficient Method for Content-and-Text Based Image Retrieval显示文摘The combination of visual and textual information in image retrieval remarkably alleviates the semantic gap of traditional image retrieval methods,and thus it has attracted much attention recently.Image retrieval based on such a combination is usually called the content-and-text based image retrieval(CTBIR).Nevertheless,existing studies in CTBIR mainly make efforts on improving the retrieval quality.To the best of our knowledge,little attention has been focused on how to enhance the retrieval efficiency.Nowadays,image data is widespread and expanding rapidly in our daily life.Obviously,it is important and interesting to investigate the retrieval efficiency.To this end,this paper presents an efficient image retrieval method named CATIRI(content-and-text based image retrieval using indexing).CATIRI follows a three-phase solution framework that develops a new indexing structure called MHIM-tree.The MHIM-tree seamlessly integrates several elements including Manhattan Hashing,Inverted index,and M-tree.To use our MHIM-tree wisely in the query,we present a set of important metrics and reveal their inherent properties.Based on them,we develop a top-k query algorithm for CTBIR.Experimental results based on benchmark image datasets demonstrate that CATIRI outperforms the competitors by an order of magnitude. | Mengqi Zeng Bin Yao Zhi-Jie Wang Yanyan Shen Feifei Li Jianfeng Zhang Hao Lin Minyi Guo | 2019 | Journal of Computer Science & Technology2019，34，2： | 0 |
| 13 | Low-temperature synthesis of sp^2 carbon nanomaterials显示文摘sp^2 carbon nanomaterials are mainly composed of sp^2-hybridized carbon atoms in the form of a hexagonal network. Due to the p bonds formed by unpaired electrons, sp^2 carbon nanomaterials possess excellent electronic, mechanical, and optical properties, which have attracted great attention in recent years.As the advanced sp^2 carbon nanomaterials, graphene and carbon nanotubes(CNTs) have great potential in electronics, sensors, energy storage and conversion devices, etc. The low-temperature synthesis of graphene and CNTs are indispensable to promote the practical industrial application. Furthermore, graphene and CNTs can even be expected to directly grow on the flexible plastic that cannot bear high temperature,expanding bright prospects for applications in emerging flexible nanotechnology. An in-depth understanding of the formation mechanism of sp^2 carbon nanomaterials is beneficial for reducing the growth temperature and satisfying the demands of industrial production in an economical and low-cost way. In this review, we discuss the main strategies and the related mechanisms in low-temperature synthesis of graphene and CNTs, including the selection of precursors with high reactivity, the design of catalyst, and the introduction of additional energy for the pre-decomposition of precursors. Furthermore, challenges and outlooks are highlighted for further progress in the practical industrial application. | Yu Ding Mengqi Zeng Lei Fu | 2019 | Science Bulletin2019，64，24： | 0 |
| 14 | Curvature geometry in 2D materials显示文摘The two-dimensional(2D)material family can be regarded as the extreme externalization form of the matter in the planar 2D space.These atomically thin materials have abundant curvature structures,which will significantly affect their atomic configurations and physicochemical properties.Curvature engineering offers a new tuning freedom beyond the thoroughly studied layer number,grain boundaries,stacking order,etc.The precise control of the curvature geometry in 2D materials can redefine this material family.Special attention will be given to this emerging field and highlight possible future directions.With the step-by-step achievement in understanding the curvature engineering effect in 2D materials and establishing reliable delicate curvature controlling strategies,a brand-new era of 2D materials research could be developed. | Nan Wei Yiran Ding Jiaqian Zhang Linyi Li Mengqi Zeng Lei Fu | 2023 | National Science Review2023，10，8： | 0 |
| 15 | General synthesis of 2D rare-earth oxide single crystals with tailorable facets显示文摘Two-dimensional(2D)rare-earth oxides(REOs)are a large family of materials with various intriguing applications and precise facet control is essential for investigating new properties in the 2D limit.However,a bottleneck remains with regard to obtaining their 2D single crystals with specific facets because of the intrinsic non-layered structure and disparate thermodynamic stability of different facets.Herein,for the first time,we achieve the synthesis of a wide variety of high-quality 2D REO single crystals with tailorable facets via designing a hard-soft-acid-base couple for controlling the 2D nucleation of the predetermined facets and adjusting the growth mode and direction of crystals.Also,the facet-related magnetic properties of 2D REO single crystals were revealed.Our approach provides a foundation for further exploring other facet-dependent properties and various applications of 2D REO,as well as inspiration for the precise growth of other non-layered 2D materials. | Linyang Li Fangyun Lu Wenqi Xiong Yu Ding Yangyi Lu Yao Xiao Xin Tong Yao Wang Shuangfeng Jia Jianbo Wang Rafael GMendes Mark HRümmeli Shengjun Yuan Mengqi Zeng Lei Fu | 2022 | National Science Review2022，9，5： | 0 |
| 16 | Synthesis of Meta Symmetric 1T'-WTe2 Using an Edge-Induced Mechanism显示文摘Lattice symmetry is vital to the properties of two-dimensional(2D)materials,yet their fixed symmetry cannot meet the increasing requirements in highly eficient and programmable electrical transport.If the structural diversity of 2D materals,as demon-strated by 1T'-WTez,is improved without any phase transition or structural reconstruction,excellent metallic 1T'-WTez would be possibly used for inte-grated devices.Here,we realized meta symmetry of 1T'-WTez by using an edge-induced mechanism,which is recognized as the combination of the intrin-sic C2v symmetry and sixfold axes.On account of the dynamically controlled growth,the meta symmetric 1T'-WTez with^94.9%purity is obtained for the first time.Meta symmetry will also keep the intrinsic electrical properties of 1T'-WTez over the node.Such meta symmetry could not only enrich the structural diversity of 1T'-WTez,but also be extended to other low-symmetry 2D materials,which would be promising for customized circuits and devices. | Yao Xiao Mengyue Zhou Jinglu Liu Bin Wei Shuanglin Yue Yuan Zhou Kena Yang Tao Zhang Mengqi Zeng Zhongchang Wang Lei Fu | 2020 | Chinese Journal of Chemistry2020，38，7： | 0 |
| 17 | Molecular Scaffold Growth of Two-Dimensional, Strong Interlayer-Bonding-Layered Materials显示文摘Currently,most two-dimensional(2D)materials that are of interest to emergent applications have focused on van der Waals–layered materials(VLMs)because of the ease with which the layers can be separated(e.g.,graphene).Strong interlayer-bonding-layered materials(SLMs)in general have not been thoroughly explored,and one of the most critical present issues is the huge challenge of their preparation,although their physicochemical proper-ty transformation should be richer than VLMs and deserves greater attention.MAX phases are a classi-cal kind of SLM. | Mengqi Zeng Yunxu Chen Enze Zhang Jiaxu Li Rafael G.Mendes Xiahan Sang Shulin Luo Wenmei Ming Yuhao Fu Mao-Hua Du Lijun Zhang David S.Parker Raymond R.Unocic Kai Xiao Chenglai Wang Tao Zhang Yao Xiao Mark H,Rummeli Faxian Xiu Lei Fu | 2019 | CCS Chemistry2019，1，1： | 0 |
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