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| 1 | Recent progress in methane dehydroaromatization: From laboratory curiosities to promising technology显示文摘Direct conversion of methane to benzene or other valuable chemicals is a very promising process for the efficient application of natural gas. Compared with conversion processes that require oxidants, non-oxidative direct conversion is more attractive due to high selectivity to the target product. In this paper, an alternative route for methane dehydrogenation and selective conversion to benzene and hydrogen without the participation of oxygen is discussed. A brief review of the catalysts used in methane dehydroaromatization (MDA) is first given, followed by our current understanding of the location and the active phase of Mo species, the reaction mechanism, the mechanism of carbonaceous deposit and the deactivation of Mo/zeolite catalysts are systematically discussed. Ways to improve the catalytic activity and stability are described in detail based on catalyst and reaction as well as reactor design. Future prospects for methane dehydroaromatization process are also presented. | Shuqi Ma Xiaoguang Guo Lingxiao Zhao Susannah Scott Xinhe Bao | 2013 | Journal of Energy Chemistry2013，22，1： | 17 |
| 2 | Recent Advances of Persistent Luminescence Nanoparticles in Bioapplications显示文摘Persistent luminescence phosphors are a novel group of promising luminescent materials with afterglow properties after the stoppage of excitation.In the past decade,persistent luminescence nanoparticles(PLNPs)with intriguing optical properties have attracted a wide range of attention in various areas.Especially in recent years,the development and applications in biomedical fields have been widely explored.Owing to the efficient elimination of the autofluorescence interferences from biotissues and the ultra-long near-infrared afterglow emission,many researches have focused on the manipulation of PLNPs in biosensing,cell tracking,bioimaging and cancer therapy.These achievements stimulated the growing interest in designing new types of PLNPs with desired superior characteristics and multiple functions.In this review,we summarize the works on synthesis methods,bioapplications,biomembrane modification and biosafety of PLNPs and highlight the recent advances in biosensing,imaging and imaging-guided therapy.We further discuss the new types of PLNPs as a newly emerged class of functional biomaterials for multiple applications.Finally,the remaining problems and challenges are discussed with suggestions and prospects for potential future directions in the biomedical applications. | Shuqi Wu Yang Li Weihang Ding Letong Xu Yuan Ma Lianbing Zhang | 2020 | Nano-Micro Letters2020，12，6： | 8 |
| 3 | Control mechanism and technique of floor heave with reinforcing solid coal side and floor corner in gob-side coal entry retaining显示文摘Floor heave is the most common convergence in gob-side entry retaining.The paper analyzes the form,process and characteristics of gob-side entry retaining with the comprehensive methods of theoretical analysis,numerical simulation and the field trial.Research results present that bending and folding floor heave is the main factor in the stage of the first panel mining;squeezing and fluidity floor heave plays a great role in the stable stage of gob-side entry retaining;the combination of the former two factors affects mainly the stage of the second mining ahead;abutment pressure is a fundamental contribution to the serious floor heave of gob-side entry retaining,and sides corners of solid coal body are key part in the case of floor heave controlling of gob-side entry retaining.Floor heave of gob-side entry retaining can be significantly controlled by reinforcing sides and corners of solid coal body,and influence rules on the floor heave of gob side entry retaining of sides supporting strength and the bottom bolt orientation in solid coal side are obtained.Research results have been successfully applied in gob-side entry retaining of G20-F23070 face haulage roadway in #2 coal mine of Pingmei Group,and the field observation shows that the proposed technique is an effective way in controlling the floor heave of gob-side entry retaining. | Chen Yong Bai Jianbiao Yan Shuai Xu Ying Wang Xiangyu Ma Shuqi | 2012 | International Journal of Mining Science and Technology2012，22，6： | 6 |
| 4 | Methane dehydroaromatization with periodic CH_4-H_2 switch:A promising process for aromatics and hydrogen显示文摘Long-term stability test of Mo/HZSM-5-N catalysts(HZSM-5-N stands for nano-sized HZSM-5) in methane dehydroaromatization(MDA)reaction has been performed with periodic CH4-H2 switch at 1033-1073 K for more than 1000 h.During this test,methane conversion ranges from 13% to 16%,and mean yield to aromatics(i.e.benzene and naphthalene) exceeds 10%.N2-physisorption,XRD,NMR and TPO measurements were performed for the used Mo/HZSM-5 catalysts and coke deposition,and the results revealed that the periodic hydrogenation can effectively suppress coke deposition by removing the inert aromatic-type coke,thus ensuring Mo/HZSM-5 partly maintained its activity even in the presence of large amount of coke deposition.The effect of zeolite particle size on the catalytic activity was also explored,and the results showed that the nano-sized zeolite with low diffusion resistance performed better.It is recognized that the size effect was enhanced by reaction time,and it became more remarkable in a long-term MDA reaction even at a low space velocity. | Changyong Sun Guangzong Fang Xiaoguang Guo Yuanli Hu Shuqi Ma Tianhua Yang Jie Han Hao Ma Dali Tan Xinhe Bao | 2015 | Journal of Energy Chemistry2015，24，3： | 6 |
| 5 | Induction of seed germination in Orobanche spp.by extracts of traditional Chinese medicinal herbs显示文摘The co-evolution of Orobanche spp.and their hosts within the same environment has resulted in a high degree of adaptation and effective parasitism whereby the host releases parasite germination stimulants,which are likely to be unstable in the soil.Our objective was to investigate whether extracts from non-host plants,specifically,Chinese medicinal plants,could stimulate germination of Orobanche spp.Samples of 606 Chinese medicinal herb species were extracted with deionized water and methanol.The extracts were used to induce germination of three Orobanche species;Orobanche minor,Orobanche cumana,and Orobanche aegyptiaca.O.minor exhibited a wide range of germination responses to the various herbal extracts.O.cumana and O.aegyptiaca exhibited an intermediate germination response to the herbal extracts.O.minor,which has a narrow host spectrum,showed higher germination rates in response to different herbal extracts compared with those of O.cumana and O.aegyptiaca,which have a broader host spectrum.Methanolic extracts of many Chinese herbal species effectively stimulated seed germination among the Orobanche spp.,even though they were not the typical hosts.The effective herbs represent interesting examples of potential trap crops.Different countries can also screen extracts from indigenous herbaceous plants for their ability to induce germination of Orobanche spp.seeds.The use of such species as trap plants could diminish the global soil seed bank of Orobanche. | MA YongQing ZHANG Wei DONG ShuQi REN XiangXiang AN Yu LANG Ming | 2012 | Science China(Life Sciences)2012，55，3： | 6 |
| 6 | Optical Micro/Nano Fibers Enabled Smart Textiles for Human-Machine Interface显示文摘Wearable human-machine interface(HMI)is an advanced technology that has a wide range of applications from robotics to augmented/virtual reality(AR/VR).In this study,an optically driven wearable human-interactive smart textile is proposed by integrating a polydimethylsiloxane(PDMS)patch embedded with optical micro/nanofibers(MNF)array with a piece of textiles.Enabled by the highly sensitive pressure dependent bending loss of MNF,the smart textile shows high sensitivity(65.5 kPa^(−1))and fast response(25 ms)for touch sensing.Benefiting from the warp and weft structure of the textile,the optical smart textile can feel slight finger slip along the MNF.Furthermore,machine learning is utilized to classify the touch manners,achieving a recognition accuracy as high as 98.1%.As a proof-of-concept,a remote-control robotic hand and a smart interactive doll are demonstrated based on the optical smart textile.This optical smart textile represents an ideal HMI for AR/VR and robotics applications. | Shuqi Ma Xiaoyu Wang Pan Li Ni Yao Jianliang Xiao Haitao Liu Zhang Zhang Longteng Yu Guangming Tao Xiong Li Limin Tong Lei Zhang | 2022 | Advanced Fiber Materials2022，4，5： | 5 |
| 7 | Single optical microfiber enabled tactile sensor for simultaneous temperature and pressure measurement显示文摘The ability to sense heat and touch is essential for healthcare,robotics,and human–machine interfaces.By taking advantage of the engineerable waveguiding properties,we design and fabricate a flexible optical microfiber sensor for simultaneous temperature and pressure measurement based on theoretical calculation.The sensor exhibits a high temperature sensitivity of 1.2 nm/℃ by measuring the shift of a high-order mode cutoff wavelength in the short-wavelength range.In the case of pressure sensing,the sensor shows a sensitivity of 4.5%per kilopascal with a fast temporal frequency response of 1000 Hz owing to the strong evanescent wave guided outside the microfiber.The cross talk is negligible because the temperature and pressure signals are measured at different wavelengths based on different mechanisms.The properties of fast temporal response,high temperature,and pressure sensitivity enable the sensor for real-time skin temperature and wrist pulse measurements,which is critical to the accurate analysis of pulse waveforms.We believe the sensor will have great potential in wearable optical devices ranging from healthcare to humanoid robots. | NI YAO XIAOYU WANG SHUQI MA XINGDA SONG SHAN WANG ZHANGXING SHI JING PAN SHIPENG WANG JIANLIANG XIAO HAITAO LIU LONGTENG YU YAO TANG ZHANG ZHANG XIONG LI WEI FANG LEI ZHANG LIMIN TONG | 2022 | Photonics Research2022，10，9： | 2 |
| 8 | In-Fiber Structured Particles and Filament Arrays from the Perspective of Fluid Instabilities显示文摘In-fiber structured particles and filament array have been recently emerging,providing unique advantages of feasible fabrication,diverse structures and sophisticated functionalities.This review will focus on the progress of this topic mainly from the perspective of fluid instabilities.By suppressing the capillary instability,the uniform layered structures down to nanometers are attained with the suitable materials selection.On the other hand,by utilizing capillary instability via post-drawing thermal treatment,the unprecedent structured particles can be designed with multimaterials for multifunctional fiber devices.Moreover,an interesting filamentation instability of a stretching viscous sheet has been identified during thermal drawing,resulting in an array of filaments.This review may inspire more future work to produce versatile devices for fiber electronics,either at a single fiber level or in large-scale fabrics and textiles,simply by manipulating and controlling fluid instabilities. | Bingrui Xu Shuqi Ma Yuanzhuo Xiang Jing Zhang Meifang Zhu Lei Wei Guangming Tao Daosheng Deng | 2020 | Advanced Fiber Materials2020，2，1： | 2 |
| 9 | In situ synthesis of biomass-derived Ni/C catalyst by self-reduction for the hydrogenation of levulinic acid to γ-valerolactone显示文摘Herein,we reported in situ synthesis of biomass-derived Ni/C catalyst by self-reduction with pomelo peel.Compared with the conventional method, which includes carbonization, activation, impregnation and reduction, the entire preparation process was simplified to two steps, which was more straightforward. This synthesis method was green as Ni/C can be prepared without any additional chemical and the self-reduction process was realized in N2, which can avoid using H2 thus averting some problems such as storage, transportation and safety of H2. Meanwhile, the size and dispersion of Ni particles can be controlled by changing carbonization temperature.The synthesis mechanism of Ni/C catalyst with selfreduction was investigated, which was mainly attributed to the carbon and reducing gas produced during the carbonization process.For the catalytic performance of GVL synthesis, a high yield (94.5%) can be obtained and it exhibited good stability up to 5 cycles without obvious loss of catalytic activity. | Shuqi Fang Zhibing Cui Yuting Zhu Chenguang Wang Jing Bai Xinghua Zhang Ying Xu Qiying Liu Lungang Chen Qi Zhang Longlong Ma | 2019 | Journal of Energy Chemistry2019，28，10： | 1 |
| 10 | Robust hydrogel sensors for unsupervised learning enabled sign-to-verbal translation显示文摘Highly stretchable and robust strain sensors are rapidly emerging as promising candidates for a diverse of wearable electronics.The main challenge for the practical application of wearable electronics is the energy consumption and device aging.Energy consumption mainly depends on the conductivity of the sensor,and it is a key factor in determining device aging.Here,we design a liq-uid metal(LM)-embedded hydrogel as a sensing material to overcome the bar-rier of energy consumption and device aging of wearable electronics.The sensing material simultaneously exhibits high conductivity(up to 22 S m�1),low elastic modulus(23 kPa),and ultrahigh stretchability(1500%)with excel-lent robustness(consistent performance against 12000 mechanical cycling).A motion monitoring system is composed of intrinsically soft LM-embedded hydrogel as sensing material,a microcontroller,signal-processing circuits,Bluetooth transceiver,and self-organizing map developed software for the visu-alization of multi-dimensional data.This system integrating multiple functions including signal conditioning,processing,and wireless transmission achieves monitor hand gesture as well as sign-to-verbal translation.This approach provides an ideal strategy for deaf-mute communicating with normal people and broadens the application of wearable electronics. | Hude Ma Haiyang Qin Xiao Xiao Na Liu Shaolei Wang Junye Li Sophia Shen Shuqi Dai Mengmeng Sun Peiyi Li Xiaofang Pan Mingjun Huang Baoyang Lu Jun Chen Lidong Wu | 2023 | InfoMat2023，5，7： | 1 |
| 11 | Environmental surveillance of SARS-CoV-2 RNA in wastewater systems and related environments in Wuhan:April to May of 2020显示文摘Wastewater-based epidemiology(WBE)has emerged as an effective environmental surveillance tool in monitoring fecal-oral pathogen infections within a community.Congruently,SARS-Co V-2,the etiologic agent of COVID-19,has been demonstrated to infect the gastrointestinal tissues,and be shed in feces.In the present study,SARS-Co V-2 RNA was concentrated from wastewater,sludge,surface water,ground water,sediment,and soil samples of municipal and hospital wastewater systems and related environments in Wuhan during the COVID-19 middle and low risk periods,and the viral RNA copies quantified using reverse transcription quantitative polymerase chain reaction(RT-q PCR).From the findings of this study,during the middle risk period,one influent sample and three secondary effluents collected from waste water treatment plant 2,as well as two samples from Jinyintan Hospital wastewater system influent were SARS-Co V-2 RNA positive.One sludge sample collected from Guanggu Branch of Tongji Hospital,which was obtained during the low risk period,was also positive for SARS-Co V-2 RNA.These study findings demonstrate the significance of WBE in continuous surveillance of SARS-Co V-2 at the community level,even when the COVID-19 prevalence is low.Overall,this study can be used as an important reference for contingency management of wastewater treatment plants and COVID-19 prevention and control departments of Wuhan. | Lu Zhao Evans Atoni Raphael Nyaruaba Yao Du Huaiyu Zhang Oscar Donde Doudou Huang Shuqi Xiao Nanjie Ren Teng Ma Zhu Shu Zhiming Yuan Lei Tong Han Xia | 2022 | Journal of Environmental Sciences2022，34，2： | 1 |
| 12 | Effectiveness of ten commercial maize cultivars in inducing Egyptian broomrape germination显示文摘Egyptian broomrape(EB),Phelipanche aegyptiaca,is a devastating root parasite,causing enormous crop losses around the world.Maize has the potential to influence the growth of other plants through releasing certain allelochemicals and is able to induce germination of at least three broomrape species.To determine whether maize could be used as a trap crop for EB,10 maize cultivars were tested for their ability to induce EB germination.The results showed that maize cultivars can induce EB germination,and that germination rates in a cut-root experiment and a hydroponic experiment were consistent.Maize cvs Changcheng 799 and Zhengdan 958 induced the highest EB germination rates,while cvs Luyu 13 and Zhengyu 203 were the least effective.These four maize cultivars were further studied in a pot experiment.Rhizosphere soil,rhizosphere soil extracts,root extracts and shoot extracts from these cultivars were all able to induce EB germination,with cv.Changcheng 799 inducing the highest germination rates.Root extracts generally induced higher germination rates than shoot extracts.It is suggested that Changcheng799 could be planted as a trap crop for control of EB. | Xiaoxin YE Jinnan JIA Yongqing MA Yu AN Shuqi DONG | 2016 | Frontiers of Agricultural Science and Engineering2016，3，2： | 1 |
| 13 | Screening of Some Cotton Varieties for Allelopathic Potential on Clover Broomrape Germination显示文摘 | Ma Yongqing Lang Ming Dong Shuqi Shui Junfeng Zhao Junxin | 2012 | EN2012，，3： | 1 |
| 14 | Fighting for the poverty:a case study for human migration in the context of sustainable dryland farming development in the Southern Ningxia Hilly Area显示文摘The Southern Ningxia Hilly Area is one of the most impoverished areas of Ningxia Hui Autonomous Region(a province)of China due to an economy that mainly relies on agriculture,which is affected by droughts in two out of every three years.Government programs have attempted to develop an increased and sustainable level of scientifically based agricultural production while restoring the environment.However,since the population exceeds the capacity of the land to adequately support it,a program is underway to move 350000 people to more suitable locations.This paper outlines the past improvements to the Southern Ningxia Hilly Area and considers future development in the context of migration for ecological reasons. | Yongqing MA Jie CHEN Shuqi DONG Lun SHAN | 2014 | Frontiers of Agricultural Science and Engineering2014，1，1： | 0 |
| 15 | A multiple flame-retardant,early fire-warning,and highly sensitive thread-shaped all-fabric-based piezoresistive sensor显示文摘In the artificial intelligence age,multifunctional and intelligent fireproof fabric-based electronics are urgently needed.Herein,a novel thread-shaped all-fabric-based piezoresistive sensor(denoted as TAFPS)with properties such as flame retardancy,firewarning,and piezoresistivity is proposed,which is composed of an inner nickel-plated fabric electrode,a multifunctional double helix fabric,and an external flame-retardant encapsulation fabric.Owing to the multiple flame-retardant properties of glass fiber tubular fabric,aminated carbon nanotubes(ACNTs),and ammonium polyphosphate,the char residue of the TAFPS reaches40.3 wt%at 800℃.In addition,the heat-sensitive effect of ACNTs during combustion causes a rapid decrease in the TAFPS resistance,triggering the fire alarm system within 2 s.Additionally,benefiting from the force-sensitive behavior of the double helix layer and tightly wrapped pattern of the external heat-shrinkable tubular fabric,TAFPS demonstrated a high sensitivity of4.40 kPa^(-1)(0–5.81 k Pa)and good stability for 10000 s.Considering its excellent flame resistance,high sensitivity,and agreeable stability,the developed TAFPS can be integrated into fire suits to monitor the exercise training process and the external fire environment.This work offers a novel approach for fabricating all-fabric-based piezoresistive sensors in the future for fire prevention and fire alarms,with promising applications in fire protection,the Internet of Things,and smart apparel. | LI WeiBiao ZHANG Shuai MA ShuQi WANG JiaCheng WANG Huan YANG QiRong SONG YongTao ZHU Jie | 2024 | Science China(Technological Sciences)2024，67，4： | 0 |
| 16 | SARS-CoV-2 spike host cell surface exposure promoted by a COPI sorting inhibitor显示文摘Via an insufficient coat protein complex I(COPI)retrieval signal,the majority of SARSCo V-2 spike(S)is resident in host early secretory organelles and a tiny amount is leaked out in cell surface.Only surface-exposed S can be recognized by B cell receptor(BCR)or anti-S therapeutic monoclonal antibodies(m Abs)that is the trigger step for B cell activation after S m RNA vaccination or infected cell clearance by S m Abs.Now,a drug strategy to promote S host surface exposure is absent.Here,we first combined structural and biochemical analysis to characterize S COPI sorting signals.A potent S COPI sorting inhibitor was then invented,evidently capable of promoting S surface exposure and facilitating infected cell clearance by S antibody-dependent cellular cytotoxicity(ADCC).Importantly,with the inhibitor as a probe,we revealed Omicron BA.1 S is less cell surface exposed than prototypes because of a constellation of S folding mutations,possibly corresponding to its ER chaperone association.Our findings not only suggest COPI is a druggable target against COVID-19,but also highlight SARS-Co V-2 evolution mechanism driven by S folding and trafficking mutations. | Yiqun Li Mingrui Yang Yanan Nan Jiaming Wang Sanjiao Wang Dongxiao Cui Jiajian Guo Pengfei He Wenxin Dai Shuqi Zhou Yue Zhang Wenfu Ma | 2023 | Acta Pharmaceutica Sinica B2023，13，7： | 0 |
| 17 | Acoustic spin-1 Weyl semimetal显示文摘The study of topological semimetals hosting spin-1 Weyl points(WPs)beyond Dirac points and WPs has attracted a great deal of attention.However,a spin-1 Weyl semimetal that exclusively possesses spin-1 WPs in a clean frequency window without being shadowed by any other nodal points is yet to be discovered.This study reports a spin-1 Weyl semimetal in a phononic crystal.Its spin-1 WPs are touched by two linear dispersions and an additional flat band and carry monopole charges(-2,0,2)or(2,0,-2)for the three bands from the bottom to the top.They result in double Fermi arcs,which occur between the first and second bands,as well as between the second and third bands.Further robust propagation is observed against the multiple joints and topological negative refraction of the acoustic surface arc wave.The results of this study create the basis for the exploration of the unusual properties of spin-1 Weyl physics on a macroscopic scale. | WeiYin Deng XueQin Huang JiuYang Lu Feng Li JiaHong Ma ShuQi Chen ZhengYou Liu | 2020 | Science China(Physics,Mechanics & Astronomy)2020，63，8： | 0 |
| 18 | The Haircare Efficacy Research of Prinsepia Utilis OilPrinsepia Oil显示文摘To research the hair-care efficacy of prinsepia utilis oil.We evaluated the haircare efficacies of prinsepia utilis oil through methods such as differential scanning calorimetry(DSC),measuring difficulty level and mechanical resistance against combing of wet and dry hair,scanning electron microscopy(SEM).According to the analysis of differential scanning calorimetry(DSC),the testing sample has repairing effect on the hairα-keratin damage induced by heated blowing.According to the pictures of scanning electron microscopy(SEM),The test results indicate the repairing or resisting thermal damage effects induced by hair drier of prinsepia utilis oil.By comparison with the blank control group,the strength and work of dry comb and wet comb were significantly reduced in the samples tested with 2%prinsepia utilis oil concentration(P﹤0.05).This indicates the testing sample has the efficacy to improve the easiness of combing and anti-tangle.And friction work is significantly reduced This indicates the smoothing efficacy of the testing sample.and the hair scales status is better;this indicates hair scales repairing efficacy of testing sample.Conclusion:PRINSEPIA UTILIS OIL has the effect of repairing hair scales,resisting thermal damage caused by hair dryer,easy to comb,anti-tangle,smoothing. | Cai Bindi Zhang Shaonuan Lu Shuqi Zhou Ji Ma Zhanlin | 2023 | China Detergent & Cosmetics2023，8，4： | 0 |
| 19 | Structural mechanism of a dual-functional enzyme Dgp A/B/C as both a C-glycoside cleaving enzyme and an O-to C-glycoside isomerase显示文摘The C-glycosidic bond that connects the sugar moiety with aglycone is difficult to be broken or made due to its inert nature.The knowledge of C-glycoside breakdown and synthesis is very limited.Recently,the enzyme Dgp A/B/C cascade from a human intestinal bacterium PUE was identified to specifically cleave the C-glycosidic bond of puerarin(daidzein-8-C-glucoside).Here we investigated how puerarin is recognized and oxidized by Dgp A based on crystal structures of Dgp A with or without substrate and biochemical characterization.More strikingly,we found that apart from being a C-glycoside cleaving enzyme,Dgp A/B/C is capable of efficiently converting O-to C-glycoside showing the activity as a structure isomerase.A possible mechanistic model was proposed dependently of the simulated complex structure of Dgp B/C with 3’’-oxo-daidzin and structure-based mutagenesis.Our findings not only shed light on understanding the enzyme-mediated C-glycosidic bond breakage and formation,but also may help to facilitate stereospecific C-glycoside synthesis in pharmaceutical industry. | Pengfei He Sha Wang Sen Li Siqi Liu Shuqi Zhou Jing Wang Jiayue Tao Dongdong Wang Rufeng Wang Wenfu Ma | 2023 | Acta Pharmaceutica Sinica B2023，13，1： | 0 |
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