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| 1 | One-step laser induced conversion of a gelatin-coated polyimide film into graphene:Tunable morphology,surface wettability and microsupercapacitor applications显示文摘Latest advances have witnessed the laser induction process on polyimide(PI)films for the formation of porous graphene.Herein,a fully converted graphene film was prepared by Nd:YAG laser scribing a gelatin coated PI film.It was found that the gelatin played the role of'shield'well in absorbing intense laser impact and benefit for the surface morphology modulation.Laser treatment lower than a critical fluence point of~4.00 J mm^(-2) contributed to a crater-like surface morphology due to the dispersed nature of Nd:YAG laser beam.By tuning laser fluence above the threshold,carbonized surface turned into continuous morphology.A fluid dynamics process accompanied by outgassing occurred during the carbonization,and the surface morphology gradually varied from stretched droplets to porous strips and finally to amorphous porous structures.The morphology evolution in combination with surface chemistry is responsible for the significant wettability transition from superhydrophobic to superhydrophilic,and a Janus superhydrophobic/superhydrophilic surface wettability was achieved under a laser fluence of~8.00 J mm^(-2).Eventually,microsupercapacitors(MSCs)were fabricated to show the great potential of our prepared graphene in flexible electronics. | WANG WenTao LU LongSheng XIE YingXi LI ZeHong WU WeiBin LIANG RongXuan TANG Yong | 2021 | Science China(Technological Sciences)2021，64，5： | 2 |
| 2 | Controlling the laser induction and cutting process on polyimide films for kirigami-inspired supercapacitor applications显示文摘The recently emerging laser-induced graphene(LIG)technology,with one-step processing and designable features,has been widely used in the fabrication of wearable/portable electronics.Herein,by taking inspiration from kirigami,we designed a stretchable supercapacitor(SC)step by step through controlling laser induction and cutting process on the polyimide(PI)film,with the use of one single CO_(2) laser source.Firstly,the carbonized basic geometric units of lines were produced on PI films to investigate the processing-structure relationships.Then,the complex photothermal conversion and heat transfer progress involved in the carbonized process were simulated by a photothermal model.Both experimental and theoretical results suggested that the laser power,scan rate and focus condition have great influence on the size,shape and morphology of the carbonized lines.Finally,we optimized the parameters of laser induction and cutting process to fabricate the kirigami-inspired SCs with reliable electrochemical properties and editable mechanical flexibility,showing great potential in the field of flexible electronics. | WANG WenTao LU LongSheng XIE YingXi WU WeiBin LIANG RongXuan LI ZeHong TANG Yong | 2021 | Science China(Technological Sciences)2021，64，3： | 2 |
| 3 | Characteristics and Formation Mechanism for Stainless Steel Fiber with Periodic Micro-fins显示文摘Metal fibers have been widely used in many industrial applications due to their unique advantages. In certain applications, such as catalyst supports or orthopedic implants, a rough surface or tiny outshoots on the surface of metal fibers to increase surface area are needed. However, it has not been concerned about the surface morphologies of metal fiber in the current research of metal fiber manufacturing. In this paper, a special multi-tooth tool composed of a row of triangular tiny teeth is designed. The entire cutting layer of multi-tooth tool bifurcates into several thin cutting layers due to tiny teeth involved in cutting. As a result, several stainless steel fibers with periodic micro-fins are produced simultaneously. Morphology of periodic micro-fins is found to be diverse and can be classified into three categories: unilateral plane, unilateral tapering and bilateral. There are two forming mechanisms for the micro-fins. One is that periodic burrs remained on the free side of cutting layer of a tiny tooth create micro-fins of stainless steel fiber produced by the next neighboring tiny tooth; the other is that the connections between two fibers stuck together come to be micro-fins if the two fibers are finally detached. Influence of cutting conditions on formation of micro-fins is investigated. Experimental results show that cutting depth has no significant effect on micro-fin formation, high cutting speed is conducive to micro-fin formation, and feed should be between 0.12 mm/r and 0.2 mm/r to reliably obtain stainless steel fiber with micro-fins. This research presents a new pattern of stainless steel fiber characterized by periodic micro-fins formed on the edge of fiber and its manufacturing method. | TANG Tao WAN Zhenping LU Longsheng TANG Yong | 2016 | Chinese Journal of Mechanical Engineering2016，29，3： | 1 |
| 4 | Anti-gravity loop-shaped heat pipe with graded pore-size wick 显示文摘 | Tang Yong Zhou Rui Lu Longsheng Xie Zichun | 2012 | Applied Thermal Engineering2012，36，： | 1 |
| 5 | Experimental investigation on capillary force of composite wick structure by IR thermal imaging camera显示文摘 | Tang Yong Deng Daxiang Lu Longsheng | 2010 | Experimental Thermal and Fluid Science2010，34，2： | 1 |
| 6 | Slave rotation analysis of miniature inner grooved copper tube through rotary swaging process显示文摘 | Lu Longsheng Yuan Dong Tang Yong | | 0，，1： | 1 |
| 7 | Laser micro-milling of microchannel on copper sheet as catalyst support used in microreactor for hydrogen production显示文摘 | ZHOU Wei DENG Wenjun LU Longsheng | 2014 | International Journal of Hydrogen Energy2014，39，10： | 1 |
| 8 | An easy-to-implement method for fabricating superhydrophobic surfaces inspired by taro leaf显示文摘An easy-to-implement method by which to fabricate superhydrophobic surfaces inspired taro leaf was successfully applied on316 L stainless steel via combining nanosecond laser(NL)processing and spin-coating techniques.The laser-textured surface composed of microscale frameworks and central bumps was fabricated by NL processing based on properly designed biomimetic patterns,and a layer of nanoscale carbon black/polydimethylsiloxane(CB/PDMS)particles was covered on it by spin-coating.The effect of pattern parameters(i.e.,the inscribed circle radius of framework and the radius of central bump)on wettability of biomimetic surface was investigated.All as-prepared biomimetic surfaces with micro-nano hierarchical structures showed excellent superhydrophobicity with the water contact angle of~155°and contact angle hysteresis of~2°.By comparing the untreated surface,the wetting behavior and evaporation mode of the biomimetic surface occurred an obvious transformation.Meanwhile,experiments indicated that the biomimetic surface not only had liquid-repelling and self-cleaning functions,but also maintained remarkable mechanical robustness and superhydrophobic durability.The method is efficient for fabricating biomimetic superhydrophobic surfaces applied to liquid-repelling,evaporation-transforming and self-cleaning fields. | LI KaiKai LEI Jiang XIE YingXi LU LongSheng ZHANG ShaoHui ZHOU PeiYang LIANG RongXuan WAN ZhenPing TANG Yong | 2021 | Science China(Technological Sciences)2021，64，12： | 0 |
| 9 | Scorpion-inspired dual-bionic,microcrack-assisted wrinkle based laser induced graphene-silver strain sensor with high sensitivity and broad working range for wireless health monitoring system显示文摘Scorpions,through ruthless survival of the fittest,evolve the unique ability to quickly locate and hunt prey with slit receptors near the leg joints and a sharp sting on the multi-freedom tail.Inspired by this fantastic creature,we herein report a dual-bionic strategy to fabricate microcrack-assisted wrinkle strain sensor with both high sensitivity and stretchability.Specifically,laserinduced graphene(LIG)is transferred from polyimide film to Ecoflex and then coated with silver paste using the casting-andpeeling and prestretch-and-release methods.The shape-adaptive and long-range ordered geometry(e.g.,amplitude and wavelength)of dual-bionic structure is prestrain-tuned to optimize the superfast response time(~76 ms),high sensitivity(gauge factor=223.6),broad working range(70%–100%),and good reliability(>800 cycles)of scorpion-inspired strain sensor,outperforming many LIG-based materials and other bionic sensors.The alternate reconnect/disconnect behaviors of slit-organlike microcracks in the mechanical weak areas initiate tremendous resistance changes,whereas the scorpion-tail-like wrinkles act as a“bridge”connecting the adjacent LIG resistor units,enabling reversible resilience and unimpeded electrical linkages over a wide strain range.Combined with the self-developed miniaturized,flexible,and all-in-one wireless transmission system,a variety of scenarios such as large body movements,tiny pulse,and heartbeat are real-time monitored via bluetooth and displayed in the client-sides,revealing a huge promise in future wearable electronics. | Wentao Wang Longsheng Lu Xiaoyu Lu Zhanbo Liang Honghao Lin Zehong Li Xiaohua Wu Lihui Lin Yingxi Xie | 2023 | Nano Research2023，16，1： | 0 |
| 10 | Fabrication of electrospun bilayer separators for lithium-sulfur batteries:A surface and structure dual modification strategy显示文摘The severe shuttle effect problem of soluble polysulfides greatly hinders the development of long-life lithium-sulfur(Li-S)batteries,which can be improved by separator modification.This study develops a bilayer separator based on an effective surface and structure dual modification strategy.This bilayer separator(named as TCNFs/SPNFs)is constructed by the integration of a carbon-based nanofiber layer(surface modification layer)with a polymer-based nanofiber layer(structure modification layer)through a facile electrospinning process.The excellent electrolyte wettability of the nanofibers accelerates lithium-ion migration,while the good electronic conductivity of the carbon layer facilitates fast electron conduction.The TiO_(2)and SiO_(2)nanoparticles embedded in the separator provide abundant active sites for immobilizing the polysulfides.Owing to these synergistic effects,this multi-functional separator helps inhibit the shuttling problem and thus enhances the active sulfur utilization.The as-prepared battery with the TCNFs/SPNFs separator delivers significantly enhanced the electrochemical performances,producing a low capacity decay rate of 0.061%per cycle at 1 C over 1000 cycles and an admirable rate capacity of 886.7 mAh g^(-1)at 2 C.Even with a high sulfur loading of 4.8 mg cm^(-2),a remarkable areal capacity of 6.0 mAh cm^(-2)is attained.This work is believed to provide a promising strategy to develop novel separators for high-performance Li-S batteries. | XU Ming ZHANG XiaoQing YUAN Wei HUANG HongLin WU YaoPeng WAN ZhenPing LU LongSheng TANG Yong | 2022 | Science China(Technological Sciences)2022，65，12： | 0 |
| 11 | Laser-induced jigsaw-like graphene structure inspired by Oxalis corniculata Linn.leaf显示文摘The laser scribing of polyimide(PI, Kapton) film is a new, simple and effective method for graphene preparation. Moreover,the superhydrophobic surface modification can undoubtedly widen the application fields of graphene. Herein, inspired by the hydrophobic and self-cleaning properties of natural Oxalis corniculata Linn. leaves, we propose a novel bionic manufacturing method for superhydrophobic laser-induced graphene(LIG). By tailoring the geometric parameters(size, roughness and height/area ratio) and chemical composition, the three-dimensional(3D) multistage LIG, i.e., with micro-jigsaw-like and porous structure, can deliver a static water contact angle(WCA) of 153.5° ± 0.6°, a water sliding angle(WSA) of 2.5° ±0.5°, and great superhydrophobic stability lasting for 100 days(WCAs ≈ 150°). This outstanding water repellency is achieved by the secondary structure of jigsaw-like LIG, a porous morphology that traps air layers at the solid–liquid interface. The robust self-cleaning and anti-stick functions of 3D bionic and multistage LIG are demonstrated to confirm its great potential in wearable electronics. | Wentao Wang Longsheng Lu Xiaoyu Lu Zhanbo Liang Biao Tang Yingxi Xie | 2022 | Bio-Design and Manufacturing2022，5，4： | 0 |
| 12 | Optical heterodyne-Zeeman modulation magnetic rotation spectroscopic technique显示文摘Optical heterodyne detection using 500 MHz phase modulation was combined with the Zeeman modulation-magnetic rotation spectroscopy (ZM-MRS) to form a new spectroscopic technique, which effectively reduced the amplitude fluctuation from laser source and greatly improved the signal-to-noise ratio in the detection of transient molecules. | Yangqin Chen Zhiyi Bi Peipei Cai Jingxin Ding Rongjun Wang Jingjing Lu Longsheng Ma | 1999 | Chinese Science Bulletin1999，44，20： | 0 |
| 13 | High-quality Fagopyrum esculentum genome provides insights into the flavonoid accumulation among different tissues and self-incompatibility显示文摘Common buckwheat(Fagopyrum esculentum)and Tartary buckwheat(Fagopyrum tataricum),the two most widely cultivated buckwheat species,differ greatly in flavonoid content and reproductive mode.Here,we report the first high-quality and chromosome-level genome assembly of common buckwheat with 1.2 Gb.Comparative genomic analysis revealed that common buckwheat underwent a burst of long terminal repeat retrotransposons insertion accompanied by numerous large chromosome rearrangements after divergence from Tartary buckwheat.Moreover,multiple gene families involved in stress tolerance and flavonoid biosynthesis such as multidrug and toxic compound extrusion(MATE)and chalcone synthase(CHS)underwent significant expansion in buckwheat,especially in common buckwheat.Integrated multi-omics analysis identified high expression of catechin biosynthesis-related genes in flower and seed in common buckwheat and high expression of rutin biosynthesis-related genes in seed in Tartary buckwheat as being important for the differences in flavonoid type and content between these buckwheat species.We also identified a candidate key rutindegrading enzyme gene(Ft8.2377)that was highly expressed in Tartary buckwheat seed.In addition,we identified a haplotype-resolved candidate locus containing many genes reportedly associated with the development of flower and pollen,which was potentially related to self-incompatibility in common buckwheat.Our study provides important resources facilitating future functional genomics-related research of flavonoid biosynthesis and selfincompatibility in buckwheat. | Qiang He Dan Ma Wei Li Longsheng Xing Hongyu Zhang Yu Wang Cailian Du Xuanzhao Li Zheng Jia Xiuxiu Li Jianan Liu Ze Liu Yuqing Miao Rui Feng Yang Lv Meijia Wang Hongwei Lu Xiaochen Li Yao Xiao Ruyu Wang Hanfei Liang Qinghong Zhou Lijun Zhang Chengzhi Liang Huilong Du | 2023 | Journal of Integrative Plant Biology2023，65，6： | 0 |
| 14 | Wearable multilead ECG sensing systems using on-skin stretchable and breathable dry adhesives显示文摘Electrocardiogram(ECG)monitoring is used to diagnose cardiovascular diseases,for which wearable electronics have attracted much attention due to their lightweight,comfort,and long-term use.This study developed a wearablemultilead ECG sensing system with on-skin stretchable and conductive silver(Ag)-coated fiber/silicone(AgCF-S)dry adhesives.Tangential and normal adhesion to pigskin(0.43 and 0.20 N/cm2,respectively)was optimized by the active control of fiber density and mixing ratio,resulting in close contact in the electrode–skin interface.The breathableAgCF-S dry electrodewas nonallergenic after continuous fit for 24 h and can be reused/cleaned(>100 times)without loss of adhesion.The AgCF encapsulated inside silicone elastomers was overlapped to construct a dynamic network under repeated stretching(10%strain)and bending(90°)deformations,enabling small intrinsic impedance(0.3,0.1 Hz)and contact impedance variation(0.7 k)in high-frequency vibration(70 Hz).All hard/soft modules of the multilead ECG system were integrated into lightweight clothing and equipped with wireless transmission for signal visualization.By synchronous acquisition of I–III,aVR,aVL,aVF,and V4 lead data,the multilead ECG sensing system was suitable for various scenarios,such as exercise,rest,and sleep,with extremely high signal-to-noise ratios. | Yingxi Xie Longsheng Lu Wentao Wang Huan Ma | 2024 | Bio-Design and Manufacturing2024，7，2： | 0 |
| 15 | Superhydrophobic Purple Orchid Leaves:Variation in Surface Morphology During the Vegetation Stages Leading to Diversity in Wettability显示文摘Learning hydrophobic phenomena from nature is always a promising approach to design the superhydrophobic surface.Purple orchid leaf which processes superhydrophobicity is an ideal plant model,and through mimicking its structure,the surface with excellent hydrophobicity is able to be obtained.However,the unclear of the diversity in wettability during the different vegetation stages and the absence of its relation to the surface morphology limits the further enhancement of the inspired structure.Here,we analyze the wettability difference as the leaf grows from tender to mature and then to senescent.Combining with the variation of surface morphology and chemical composition,the well-developed micro-scale basic unit bumps with dense nano-scale waxy layer on the surface are proven to be responsible for the best hydrophobicity of the mature leaf.The presence of the undeveloped or damaged micro-nano hierarchical structure reduces the formation of air pockets at the interface,leading to the decrease of the wettability for leaves at other stages.Moreover,by fabricating artificial leaves,the nano-waxy layer is proved to be more effective than that of the micro-bumps on the surface wettability.The results of study are of a great significance for guiding the design and fabrication of plant-inspired bionic superhydrophobic surface. | Longsheng Lu Guoxiang Jiang Kaikai Li Yingxi Xie Jiao Gao | 2023 | Journal of Bionic Engineering2023，20，6： | 0 |
| 16 | Rational design and low-cost fabrication of multifunctional separators enabling high sulfur utilization in long-life lithium-sulfur batteries显示文摘The lithium-sulfur(Li-S)battery with an ultrahigh theoretical energy density has emerged as a promising rechargeable battery system.However,the practical applications of Li-S batteries are severely plagued by the sluggish reaction kinetics of sulfur species and notorious shuttling of soluble lithium polysulfides(LiPSs)intermediates that result in low sulfur utilization.The introduction of functional layers on separators has been considered as an effective strategy to improve the sulfur utilization in Li-S batteries by achieving effective regulation of LiPSs.Herein,a promising self-assembly strategy is proposed to achieve the low-cost fabrication of hollow and hierarchically porous Fe_(3)O_(4)nanospheres(p-Fe_(3)O_(4)-NSs)assembled by numerous extremely-small primary nanocrystals as building blocks.The rationally-designed p-Fe_(3)O_(4)-NSs are utilized as a multifunctional layer on the separator with highly efficient trapping and conversion features toward LiPSs.Results demonstrate that the nanostructured p-Fe_(3)O_(4)-NSs provide chemical adsorption toward LiPSs and kinetically promote the mutual transformation between LiPSs and Li_(2)S_(2)/Li_(2)S during cycling,thus inhibiting the LiPSs shuttling and boosting the redox reaction kinetics via a chemisorption-catalytic conversion mechanism.The enhanced wettability of the p-Fe_(3)O_(4)-NSs-based separator with the electrolyte enables fast transportation of lithium ions.Benefitting from these alluring properties,the functionalized separator with p-Fe_(3)O_(4)-NSs endows the battery with an admirable rate performance of 877 mAh g^(−1)at 2 C,an ultra-durable cycling performance of up to 2176 cycles at 1 C,and a promising areal capacity of 4.55 mAh cm^(−2)under high-sulfur-loading and lean-electrolyte conditions(4.29 mg cm^(−2),electrolyte/ratio:8μl mg^(−1)).This study will offer fresh insights on the rational design and low-cost fabrication of multifunctional separator to strengthen electrochemical reaction kinetics by regulating LiPSs conversion for developing efficient and long-life Li-S batteries. | Xiaoqing Zhang Wei Yuan Honglin Huang Ming Xu Yu Chen Bote Zhao Xinrui Ding Shiwei Zhang Yong Tang Longsheng Lu | 2023 | International Journal of Extreme Manufacturing2023，5，1： | 0 |
| 17 | Investigation on forward and backward transfer process during carbon fiber/epoxy composites dry-sliding against iron alloy显示文摘Carbon fiber reinforced polymer(CFRP)composites with high load-bearing capacity are currently ideal materials in tribological load systems.One of the unique features during the friction process of CFRP/metal is the in-situ formation of an ultrathin and uniform transfer film on the metal surface,and the related initial/transfer mechanism is very important but still unclear.Recent studies mainly focus on the one-way transfer process of CFRP to the metal surface,that is,forward transfer;whereas another easily overlooked issue is that the metal material also transfers backward to the CFRP surface.Herein,we firstly prepared carbon fiber/epoxy resin composites(CF/EP)by the hot-pressing method and then carried out friction tests with iron alloy as the control material.The underlying mechanism of the forward/backward transfer process is revealed by controlling the morphological evolution and iron content of the transfer film on worn CF/EP.According to the variation law of friction coefficient with time,the interfacial friction is divided into three different stages,among which the behaviours of“micro-convex contact”and“epoxy exfoliation”occur throughout the whole procedure.We believe this work could provide a meaningful reference for studying the friction behaviour and mechanism,especially the forward and backward transfer between composites/metals,and further broaden its emerging applications in future energy,aerospace and rail transportation. | LU LongSheng LI ZeHong FANG HeZhengZi XIE YingXi WANG WenTao | 2022 | Science China(Technological Sciences)2022，65，11： | 0 |
| 18 | Capillary Performance of Nanoporous Aluminum Braided Wicks Prepared by Anodic Oxidation显示文摘With the rapid development of two-phase heat exchangers,the further improvement of the capillary performance of their internal wick faces a great challenge.As an important technology in the surface treatment of aluminum alloys,anodic oxidation has been widely used to develop various functional nanostructures.In this study,nanopores with diameters of 30–40 nm were fabricated on the surface of aluminum fibers through anodic oxidation under an oxalic acid system.Results showed that anodizing increased the specific surface area of the aluminum braid by 163 times,and changed its surface wettability from hydrophobic to superhydrophilic.A significant reduction in the effective capillary radius can substantially increase the capillary force of aluminum braids on the basis of capillary theory.Therefore,the nanoporous aluminum braids can be used as a novel wick in the vapor chamber to improve its capillary performance.Capillary rate-of-rise tests with ethanol and acetone were performed to characterize the capillary of this novel wick structure.Infrared thermal imaging was utilized to monitor the capillary rise of aluminum braided wicks.The capillary force of the anodized wicks was greater than that of a normal wick,and the maximum capillary rise height was 81 mm.The nanoporous aluminum braided wicks prepared by anodizing could be applied in heat transfer. | Fei Gao Longsheng Lu Xiaokang Mei Yu-Xiang Yu Shitong Chai Yang Shen Yingxi Xie | 2022 | Nanomanufacturing and Metrology2022，5，4： | 0 |
| 19 | Cutting performance of surgical electrodes by constructing bionic microstriped structures显示文摘Surgical electrodes rely on thermal effect of high-frequency current and are a widely used medical tool for cutting and coagulating biological tissue.However,tissue adhesion on the electrode surface and thermal injury to adjacent tissue are serious problems in surgery that can affect cutting performance.A bionic microstriped structure mimicking a banana leaf was constructed on the electrode via nanosecond laser surface texturing,followed by silanization treatment,to enhance lyophobicity.The effect of initial,simple grid-textured,and bionic electrodes with different wettabilities on tissue adhesion and thermal injury were investigated using horizontal and vertical cutting modes.Results showed that the bionic electrode with high lyophobicity can effectively reduce tissue adhesion mass and thermal injury depth/area compared with the initial electrode.The formation mechanism of adhered tissue was discussed in terms of morphological features,and the potential mechanism for antiadhesion and heat dissipation of the bionic electrode was revealed.Furthermore,we evaluated the influence of groove depth on tissue adhesion and thermal injury and then verified the antiadhesion stability of the bionic electrode.This study demonstrates a promising approach for improving the cutting performance of surgical electrodes. | Kaikai LI Longsheng LU Huaping CHEN Guoxiang JIANG Huanwen DING Min YU Yingxi XIE | 2023 | Frontiers of Mechanical Engineering2023，18，1： | 0 |
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