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2篇 您的检索式:作者名="JunSen Xiang"
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1Generic Seebeck effect from spin entropy显示文摘How magnetism affects the Seebeck effect is an important issue of wide concern in the thermoelectric community but remains elusive.Based on a thermodynamic analysis of spin degrees of freedom on varied d-electron-based ferromagnets and antiferromagnets,we demonstrate that in itinerant or partially itinerant magnetic compounds there exists a generic spin contribution to the Seebeck effect over an extended temperature range from slightly below to well above the magnetic transition temperature.This contribution is interpreted as resulting from transport spin entropy of(partially)delocalized conducting d electrons with strong thermal spin fluctuations,even semiquantitatively in a single-band case,in addition to the conventional diffusion part arising from their kinetic degrees of freedom.As a highly generic effect,the spin-dependent Seebeck effect might pave a feasible way toward efficient“magnetic thermoelectrics.”Peijie Sun K.Ramesh Kumar Meng Lyu Zhen Wang Junsen Xiang Wenqing Zhang 2021The Innovation2021,2,2:1
2Large transverse thermoelectric figure of merit in a topological Dirac semimetal显示文摘The Seebeck effect encounters a few fundamental constraints hindering its thermoelectric(TE)conversion efficiency.Most notably,there are the charge compensation of electrons and holes that diminishes this effect,and the Wiedemann-Franz(WF)law that makes independent optimization of the corresponding electrical and thermal conductivities impossible.Here,we demonstrate that in the topological Dirac semimetal Cd3As2 the Nernst effect,i.e.,the transverse counterpart of the Seebeck effect,can generate a large TE figure of merit zNT.At room temperature,zNT≈0.5 in a small field of 2 T and it significantly surmounts its longitudinal counterpart for any field.A large Nernst effect is generically expected in topological semimetals,benefiting from both the bipolar transport of compensated electrons and holes and their high mobilities.In this case,heat and charge transport are orthogonal,i.e.,not intertwined by the WF law anymore.More importantly,further optimization of zNT by tuning the Fermi level to the Dirac node can be anticipated due to not only the enhanced bipolar transport,but also the anomalous Nernst effect arising from a pronounced Berry curvature.A combination of the topologically trivial and nontrivial advantages promises to open a new avenue towards high-efficient transverse thermoelectricity.JunSen Xiang SiLe Hu Meng Lyu WenLiang Zhu ChaoYang Ma ZiYu Chen Frank Steglich GenFu Chen PeiJie Sun 2020Science China(Physics,Mechanics & Astronomy)2020,63,3:0
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