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| 1 | Zirconium-containing UiO-66 as an efficient and reusable catalyst for transesterification of triglyceride with methanol显示文摘Zirconium-based MOFs of the UiO family have attracted considerable attention due to their high thermal,chemical and mechanical stability. With the aim of further exploring the applications of zirconium-based UiO-66 in acid-catalyzed reactions and elucidating the effects of the defects in UiO-66 materials on their catalytic performances, in this work, a series of zirconium-containing UiO-66 samples were synthesized by varying the synthesis temperatures and BDC/Zr(terephthalic acid/ZrCl_4) ratios in the synthesis system.The synthesized UiO-66 samples were characterized by X-ray diffraction(XRD), N_2 adsorption-desorption,scanning electron microscopy(SEM), thermogravimetrical analysis(TGA), temperature-programmed desorption of NH_3(NH_3-TPD). Their catalytic performances were investigated in transesterification of tributyrin and soybean oil with methanol. The results showed that UiO-66 samples with different amounts of defects could be successfully prepared by varying the synthesis temperatures and/or the BDC/Zr ratios used in the synthesis system. The catalytic activities of the UiO-66 materials greatly depended on their linker defects and enhanced with the increase of the defect amount. The UiO-66 was an efficient catalyst for transesterification of tributyrin and soybean oil with methanol under mild reaction conditions and its catalytic activity was comparable to other solid acid catalysts reported in the literatures. The UiO-66 catalyst was relatively stable and could be reused. | Fan Zhou Ningyue Lu Binbin Fan Huigang Wang Ruifeng Li | 2016 | Journal of Energy Chemistry2016，25，5： | 6 |
| 2 | Clemastine rescues behavioral changes and enhances remyelination in the cuprizone mouse model of demyelination显示文摘Increasing evidence suggests that white matter disorders based on myelin sheath impairment may underlie the neuropathological changes in schizophrenia.But it is unknown whether enhancing remyelination is a beneficial approach to schizophrenia.To investigate this hypothesis,we used clemastine,an FDA-approved drug with high potency in promoting oligodendroglial differentiation and myelination,on a cuprizone-induced mouse model of demyelination.The mice exposed to cuprizone(0.2%in chow) for 6 weeks displayed schizophrenia-like behavioral changes,including decreased exploration of the center in the open field test and increased entries into the arms of the Y-maze,as well as evident demyelination in the cortex and corpus callosum.Clemastine treatment was initiated upon cuprizone withdrawal at 10 mg/kg per day for3 weeks.As expected,myelin repair was greatly enhanced in the demyelinated regions with increased mature oligodendrocytes(APC-positive) and myelin basic protein.More importantly,the clemastine treatment rescued the schizophrenia-like behavioral changes in the open field test and the Y-maze compared to vehicle,suggesting a beneficial effect via promoting myelin repair.Our findings indicate that enhancing remyelination may be a potential therapy for schizophrenia. | Zhifang Li Yangtao He Shuangyi Fan Binbin Sun | 2015 | Neuroscience Bulletin2015，31，5： | 4 |
| 3 | A stepwise-designed Rh-Au-Si nanocomposite that surpasses Pt/C hydrogen evolution activity at high overpotentials显示文摘由 electrocatalysis 的氢进化是供应干净精力的一个吸引人的方法。然而,它正在质问发现稀罕、昂贵的铂的便宜、有效的选择基于催化剂。磅提供最好的氢进化表演,因为它最佳地平衡吸附和解吸附作用的免费精力。这些数量的适当控制为生产有效 electrocatalyst 是必要的。我们示威,基于第一原则计算,逐步的设计 Rh-Au-Si 第三的催化剂,吸附(Volmer 反应) 和解吸附作用(Heyrovsky 反应) 在发生在 Rh 和 Si 上分别地出现。中间的 Au 表面由从 Rh 把氢散开提升到 Si 表面起一个重要作用。理论预言广泛地被探索了并且由试验性的观察验证了。优化催化剂(Rh-Au-SiNW-2 ) 有 2.2:28.5:69.3 的一篇作文(Rh : Au : Si 集体比率) 并且展出 24.0 mV 的一个 Tafel 斜坡 ? | Binbin Jiang Lulu Yang Fan Liao Minqi Sheng Haozhe Zhao Haiping Lin Mingwang Shao | 2017 | Nano Research2017，10，5： | 3 |
| 4 | Cuprous Oxide/Nitrogen-doped Graphene Nanocomposites as Electrochemical Sensors for Ofloxacin Determination显示文摘 | WU Fanghui XU Fan CHEN Le JIANG Binbin SUN Wenbin WEI Xianwen | 2016 | Chemical Research in Chinese Universities2016，32，3： | 3 |
| 5 | One-step synthesis of dimethyl ether from syngas on ordered mesoporous copper incorporated alumina显示文摘Ordered mesoporous copper incorporated Al_2O_3(Cu/Al_2O_3) with high Cu dispersion were prepared by a facile solution combustion synthesis method using aluminum nitrate and copper nitrate as oxidants and urea as fuel. It is a facile and green route to synthesize catalysts for dimethyl ether directly from syngas. Cu/Al_2O_3 catalysts were characterized by XRD, N_2 adsorption–desorption, SEM-EDS, and H_2-TPR.The results indicate that the catalysts obtain an ordered mesoporous structure and copper is homogenously dispersed. The mesoporous Cu/Al_2O_3 catalysts were utilized as bifunctional catalysts in syngas to dimethyl ether reaction(STD). The copper content affects the catalytic performance in STD reaction. The CO conversion and DME selectivity of Cu/Al_2O_3 with 15% copper molar ratio achieve 52.9% and 66.1%,respectively. Moreover, the mesoporous Cu/Al_2O_3 catalysts show excellent stability in STD reaction. | Yan Wang Yuexian Chen Feng Yu Dahai Pan Binbin Fan Jinghong Ma Ruifeng Li | 2016 | Journal of Energy Chemistry2016，25，5： | 3 |
| 6 | Range of ecological impact of highway construction in the Longitudinal Range-Gorge Region,China显示文摘The major features of different road sections were identified.Methods quantitatively determining the ecological impact of highway construction were discussed,and a demonstration was presented.The Dabao highway(from Dali to Baoshan)and the Sixiao highway(from Simao to Xiaomengyang)passing through the Longitudinal Range-Gorge Region were used as examples in this paper.For the normal road sections having no important species to protect,a method of ecosystem health assessment was introduced to calculate the overall range of the ecological impact of highway construction.For the road sections having plants or soils of interest,indexes were selected and the range of impact was determined using mathematical methods such as regression analysis and variance analysis.The range of impact on animal populations was also discussed in terms of the minimum living areas required by animal populations and the fragmentation caused by highway construction.The results indicate that the zones impacted by highway construction were composed of both regular and anomalous figures,the range of impacts for different landforms of the two sample highways were substantially different;highway construction had dramatic effects on roadside ecosystem health;the impact on soil factors of farmland was greater than 200 m,and the distance may exceed 1000 m when important large animals were considered. | Jie LIU Fan CHEN Haiqing GENG Xinxin QIU Binbin CAI | 2010 | Frontiers of Environmental Science & Engineering2010，4，3： | 3 |
| 7 | Enhanced Potassium‑Ion Storage of the 3D Carbon Superstructure by Manipulating the Nitrogen‑Doped Species and Morphology显示文摘Potassium-ion batteries(PIBs)are attractive for gridscale energy storage due to the abundant potassium resource and high energy density.The key to achieving high-performance and large-scale energy storage technology lies in seeking eco-efficient synthetic processes to the design of suitable anode materials.Herein,a spherical sponge-like carbon superstructure(NCS)assembled by 2D nanosheets is rationally and efficiently designed for K+storage.The optimized NCS electrode exhibits an outstanding rate capability,high reversible specific capacity(250 mAh g^(−1) at 200 mA g^(−1) after 300 cycles),and promising cycling performance(205 mAh g^(−1) at 1000 mA g^(−1) after 2000 cycles).The superior performance can be attributed to the unique robust spherical structure and 3D electrical transfer network together with nitrogen-rich nanosheets.Moreover,the regulation of the nitrogen doping types and morphology of NCS-5 is also discussed in detail based on the experiments results and density functional theory calculations.This strategy for manipulating the structure and properties of 3D materials is expected to meet the grand challenges for advanced carbon materials as high-performance PIB anodes in practical applications. | Yanhua Li Kui Xiao Cong Huang Jin Wang Ming Gao Aiping Hu Qunli Tang Binbin Fan Yali Xu Xiaohua Chen | 2021 | Nano-Micro Letters2021，13，1： | 2 |
| 8 | The solar wind plasma upstream of Mars observed by Tianwen-1:Comparison with Mars Express and MAVEN显示文摘On the great journey to Mars,China’s first planetary exploration mission,the Tianwen-1 came within 26 million kilometers of Mars from 31 October 2020 to 25 January 2021 and was getting closer to its destination,the red planet,in search of answers to the cataclysmic climate change that occurred in Martian history.Both the escape of the Martian atmosphere and the loss of surface water were firmly influenced by solar activities.Tianwen-1 provided a unique chance to depict the solar wind streams between Earth and Mars during the minimum of Solar Cycle 25.During the three-month cruise phase of Tianwen-1,the solar wind flows were successively observed at Earth,Tianwen-1,and Mars.After the field of view correction and noise reduction,the solar wind velocity and density measured by Tianwen-1 show good agreement with those at Earth and Mars.The results indicate that the performance of the ion analyzer onboard the Tianwen-1 orbiter is reliable and stable.It is worth looking forward to the joint observations of ion escape with other Mars probes in the following Martian years. | Kai FAN Limei YAN Yong WEI Aibing ZHANG Linggao KONG Markus FRÄNZ Fei HE Lihui CHAI Chongjing YUAN Yuqi WANG Jun ZHONG Zhaojin RONG Zhonghua YAO Yongxin PAN Jun CUI Jiansen HE Wenya LI Binbin TANG Chi WANG | 2022 | Science China Earth Sciences2022，65，4： | 2 |
| 9 | Polarization-independent highly efficient generation of Airy optical beams with dielectric metasurfaces显示文摘Airy optical beams have emerged to hold enormous theoretical and experimental research interest due to their outstanding characteristics.Conventional approaches suffer from bulky and costly systems,as well as poor phase discretization.The newly developed metasurface-based Airy beam generators have constraints of polarization dependence or limited generation efficiency.Here,we experimentally demonstrate a polarization-independent silicon dielectric metasurface for generation of high-efficiency Airy optical beams.In our implementation,rather than synchronous manipulation of the amplitude and phase by plasmonic or Huygens’metasurfaces,we employ and impose a 3/2 phase-only manipulation to the dielectric metasurface,consisting of an array of silicon nanopillars with an optimized transmission efficiency as high as 97%.The resultant Airy optical beams possess extraordinarily large deflection angles and relatively narrow beam widths.Our validated scheme will open up a fascinating doorway to broaden the application scenarios of Airy optical beams on ultracompact photonic platforms. | Binbin Yu Jing Wen Lei Chen Leihong Zhang Yulong Fan Bo Dai Saima Kanwal Dangyuan Lei Dawei Zhang | 2020 | Photonics Research2020，8，7： | 2 |
| 10 | Triangulation of red sprites observed above a mesoscale convective system in North China显示文摘The triangulation of red sprites was obtained, based on concurrent observations over a mesoscale convective system(MCS) in North China from two stations separated by about 450 km. In addition, broadband sferics from the sprite-producing lightning were measured at five ground stations, making it possible to locate and identify the individual causative lightning discharges for different elements in this dancing sprite event. The results of our analyses indicate that the sprites were produced above the trailing stratiform region of the MCS, and their parent strokes were located mainly in the peripheral area of the stratiform. The lateral offset between sprites and causative strokes ranges from a few km to more than 50 km. In a particularly bright sprite, with a distinct halo feature and streamers descending down to an altitude of approximately 48 km, the sprite current signal identified in the electric sferic, measured at a range of about 1,110 km, peaked at approximately 1 ms after the return stroke. | YongPing Wang GaoPeng Lu Ming Ma HongBo Zhang YanFeng Fan GuoJin Liu ZheRun Wan Yu Wang Kang-Ming Peng ChangZhi Peng FeiFan Liu BaoYou Zhu BinBin Ni XuDong Gu Long Chen Juan Yi RuoXian Zhou | 2019 | Earth and Planetary Physics2019，3，2： | 2 |
| 11 | Study on Carbonation Damage Constitutive Curve and Microscopic Damage Mechanism of Tailing Recycled Concrete显示文摘To improve the resource utilization of recycled aggregate concrete(RAC)and make use of the unique pozzolanic activation characteristics of iron ore tailing(IOT),the constitutive curves of tailing recycled concrete(TRC)before and after carbonization were analyzed theoretically,experimentally and microscopically.Firstly,according to the experimental data,the damage constitutive and related damage parameters of TRC were theoretically established by Weibull probability distribution function.Secondly,the comprehensive damage parameter b under different working conditions was studied.Finally,the damage mechanism was formed by EDS and SEM.The results showed that the damage constitutive model based on Weibull probability distribution function was in good agreement with the experimental results.Under each carbonization period,the b first decreased and then rose with the increase of tailings content.When its content was 30%,the b values of TRC were minimized,which were 22.14%,20.99%,25.39%lower than those of NAC,and 41.09%,34.89%,35.44%lower than those of RAC,indicating that IOT had a relatively good optimization effect on the constitutive curve of RAC.The microscopic analysis results also proved that the IOT addition with a proper amount would improve the matrix structure of RAC and increased its compactness,but when the content was higher,it would also cause harmful cracks in its matrix structure and reduced its density.Therefore,the optimal tailing content was about 30%.This paper provided a new method for damage constitutive calculation and analysis of TRC before and after carbonization. | Tao Li Sheliang Wang Fan Xu Binbin Li Bin Dang Meng Zhan Zhiqi Wang | 2021 | Journal of Renewable Materials2021，9，8： | 2 |
| 12 | Highly efficient synthesis of cyclic carbonates from CO 2 and epoxides catalyzed by KI/lecithin显示文摘 | Jinliang Song Binbin Zhang Peng Zhang Jun Ma Jinli Liu Honglei Fan Tao Jiang Buxing Han | 2011 | Catalysis Today2011，，1： | 1 |
| 13 | The C_(6)D_(6)detector system on the Back-n beam line of CSNS显示文摘Introduction The neutron capture cross sections are very important in the field of nuclear device design and basic physics research.Hydrogen-free liquid scintillator such as C_(6)D_(6)detectors are widely used in the neutron capture cross-sectional measurements for the low neutron sensitivity and fast time response.The Back-n white neutron source at China Spallation Neutron Source is the first spallation white neutron source in China,and it is suitable for neutron capture cross-sectional measurement.Materials and methods A C_(6)D_(6)detector system was built in the Back-n experimental station.The pulse height weighting technique was used to determine the system’s detection efficiency.The response to gamma rays of the C_(6)D_(6)detector was measured,and the energy resolution function was determined.Monte Carlo simulation with Geant4 code was carried out to get the weighting function of this C_(6)D_(6)detector system.Additionally,the systematic uncertainty of the weighting function was also determined.Conclusion According to the experimental and simulation results,this C_(6)D_(6)detector system can be used to measure neutron capture cross section. | Jie Ren Xichao Ruan Jie Bao Guangyuan Luan Wei Jiang Qi An Huaiyong Bai Ping Cao Qiping Chen Yonghao Chen Pinjing Cheng Zengqi Cui Ruirui Fan Changqing Feng Minhao Gu Fengqin Guo Changcai Han Zijie Han Guozhu He Yongcheng He Yuefeng He Hanxiong Huang Weiling Huang Xiru Huang Xiaolu Ji Xuyang Ji Haoyu Jiang Hantao Jing Ling Kang Mingtao Kang Bo Li Lun Li Qiang Li Xiao Li Yang Li Yang Li Rong Liu Shubin Liu Xingyan Liu Yinglin Ma Changjun Ning Binbin Qi Zhaohui Song Hong Sun Xiaoyang Sun Zhijia Sun Zhixin Tan Hongqing Tang Jingyu Tang Pengcheng Wang Qi Wang Taofeng Wang Yanfeng Wang Zhaohui Wang Zheng Wang Jie Wen Zhongwei Wen Qingbiao Wu Xiaoguang Wu Xuan Wu Likun Xie Yiwei Yang Han Yi Li Yu Tao Yu Yongji Yu Guohui Zhang Jing Zhang Linhao Zhang Liying Zhang Qingmin Zhang Qiwei Zhang Xianpeng Zhang Yuliang Zhang Zhiyong Zhang Yingtan Zhao Liang Zhou Zuying Zhou Danyang Zhu Kejun Zhu Peng Zhu | 2019 | Radiation Detection Technology and Methods2019，3，3： | 1 |
| 14 | Hypoxia-ischemic encephalopathy in full-term neonate: correlation proton MR spectroscopy with MR imaging显示文摘 | Guoguang Fan Zhenhua Wu Liying Chen Qiyong Guo Binbin Ye Jian Mao | 2002 | European Journal of Radiology2002，，： | 1 |
| 15 | Polymorphisms in genes of APE1 , PARP1 , and XRCC1 : risk and prognosis of colorectal cancer in a Northeast Chinese population显示文摘 | Ye Li Shuying Li Zhiwei Wu Fulan Hu Lin Zhu Xiaojuan Zhao Binbin Cui Xinshu Dong Suli Tian Fan Wang Yashuang Zhao | 2013 | Medical Oncology2013，，2： | 1 |
| 16 | Synthesis and characterization of NaY-encapsulated CuCl14Pc prepared by CuCl14Pc-containing solid gel显示文摘 | Fan Binbin Li Ruifeng Fan Weibin | 2000 | Journal of Natural Gas Chemistry2000，9，2： | 1 |
| 17 | In Situ Prepara- tion of Functional Heterogeneous Organotin Catalyst Tethered on SBA-15显示文摘 | Fan Binbin Zhang Jilong Li Ruifeng | 2008 | Catal Lett2008，121，34： | 1 |
| 18 | Organotin Com- pounds Immobilized on Mesoporous Silicas as Heterogeneous Catalysts for Direct Synthesis of Dimethyl Carbonate from Methanol and Carbon Dioxide显示文摘 | Fan Binbin Li Hongyu Fan Weibin | 2010 | Appl Catal A2010，372，1： | 1 |
| 19 | Development of a UFLC–MS/MS method for simultaneous determination of six lignans of Schisandra chinensis (Turcz.) Baill. in rat plasma and its application to a comparative pharmacokinetic study in normal and insomnic rats显示文摘 | Binbin Wei Qing Li Dan Su Ronghua Fan Longshan Zhao Lulu Geng Bosai He Xiaohui Chen Ying Jia Kaishun Bi | 2013 | Journal of Pharmaceutical and Biomedical Analysis2013，，： | 1 |
| 20 | New Gene Variants Associated with the Risk of Chronic HBV Infection显示文摘Some patients with chronic hepatitis B virus(HBV)infection failed to clear HBV,even persistently continue to produce antibodies to HBV.Here we performed a two stage genome wide association study in a cohort of Chinese patients designed to discover single nucleotide variants that associate with HBV infection and clearance of HBV.The first stage involved genome wide exome sequencing of 101 cases(HBsAg plus anti-HBs positive)compared with 102 control patients(antiHBs positive,HBsAg negative).Over 80%of individual sequences displayed 209 sequence coverage.Adapters,uncertain bases[10%or low-quality base calls([50%)were filtered and compared to the human reference genome hg19.In the second stage,579 chronic HBV infected cases and 439 HBV clearance controls were sequenced with selected genes from the first stage.Although there were no significant associated gene variants in the first stage,two significant gene associations were discovered when the two stages were assessed in a combined analysis.One association showed rs506121-“T”allele[within the dedicator of cytokinesis 8(DOCK8)gene]was higher in chronic HBV infection group than that in clearance group(P=0.002,OR=0.77,95%CI[0.65,0.91]).The second association involved rs2071676—A allele within the Carbonic anhydrase(CA9)gene that was significantly elevated in chronic HBV infection group compared to the clearance group(P=0.0003,OR=1.35,95%CI[1.15,1.58]).Upon replication these gene associations would suggest the influence of DOCK8 and CA9 as potential risk genetic factors in the persistence of HBV infection. | Mengjie Fan Jing Wang Sa Wang Tengyan Li Hong Pan Hankui Liu Huifang Xu Daria V.Zhernakova Stephen J.O’Brien Zhenru Feng Le Chang Erhei Dai Jianhua Lu Hongli Xi Yanyan Yu Jianguo Zhang Binbin Wang Zheng Zeng | 2020 | Virologica Sinica2020，35，4： | 1 |
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