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| 1 | Highly efficient Ag-modified copper phyllosilicate nanotube:Preparation by co-ammonia evaporation hydrothermal method and application in the selective hydrogenation of carbonate显示文摘Rapidly deactivation of Cu/SiO2 catalysts at high liquid hour space velocity(LHSV) has been an important obstacle for scale-up application.Herein,silver modified copper phyllosilicate nanotubes were fabricated by different strategies,and implemented to the selective hydrogenation of ethylene carbonate(EC) to methanol and ethylene glycol(EG) as alternative route for the indirect utilization of CO2.The CuPs Ag-copre catalyst synthesized by the co-ammonia evaporation hydrothermal process achieved79% methanol and 99% EG yield within various ranges of EC LHSV,which was attributed to the balanced Cu+/CuO ratio and the enhanced H2 dissociation ability.Inlaid silver species over copper phyllosilicate promoted the interaction between the metal and the support,which substantially regulated the reducibility and dispersion of copper species,meanwhile,increased the stability for long-term running of the catalyst. | Huabo Li Yuanyuan Cui Yixin Liu Lu Zhang Quan Zhang Juhua Zhang Wei-Lin Dai | 2020 | Journal of Materials Science & Technology2020，47，12： | 4 |
| 2 | Large-sized bone defect repair by combining a decalcified bone matrix framework and bone regeneration units based on photo-crosslinkable osteogenic microgels显示文摘Physiological repair of large-sized bone defects is great challenging in clinic due to a lack of ideal grafts suitable for bone regeneration.Decalcified bone matrix(DBM)is considered as an ideal bone regeneration scaffold,but low cell seeding efficiency and a poor osteoinductive microenvironment greatly restrict its application in large-sized bone regeneration.To address these problems,we proposed a novel strategy of bone regeneration units(BRUs)based on microgels produced by photo-crosslinkable and microfluidic techniques,containing both the osteogenic ingredient DBM and vascular endothelial growth factor(VEGF)for accurate biomimic of an osteoinductive microenvironment.The physicochemical properties of microgels could be precisely controlled and the microgels effectively promoted adhesion,proliferation,and osteogenic differentiation of bone marrow mesenchymal stem cells(BMSCs)in vitro.BRUs were successfully constructed by seeding BMSCs onto microgels,which achieved reliable bone regeneration in vivo.Finally,by integrating the advantages of BRUs in bone regeneration and the advantages of DBM scaffolds in 3D morphology and mechanical strength,a BRU-loaded DBM framework successfully regenerated bone tissue with the desired 3D morphology and effectively repaired a large-sized bone defect of rabbit tibia.The current study developed an ideal bone biomimetic microcarrier and provided a novel strategy for bone regeneration and large-sized bone defect repair. | Junxiang Hao Baoshuai Bai Zheng Ci Jincheng Tang Guanhuai Hu Chengxiang Dai Mengyuan Yu Meng Li Wei Zhang Yixin Zhang Wenjie Ren Yujie Hua Guangdong Zhou | 2022 | Bioactive Materials2022，7，8： | 2 |
| 3 | Application of immunosuppressant facilitates the therapy of optic neuritis combined with Sj(o)gren's syndrome显示文摘 | Li Hongyang Liu Zihao Gong Yan Jiang Zhaocai Zhang Yixin Dai Yanli Zhang Yan Wei Shihui | 2014 | Chinese Medical Journal2014，，17： | 2 |
| 4 | Injectable self-healing hydrogel with siRNA delivery property for sustained STING silencing and enhanced therapy of intervertebral disc degeneration显示文摘Inflammatory responses of nucleus pulposus(NP)can induce imbalanced anabolism and catabolism of extracellular matrix,and the cytosolic dsDNA accumulation and STING-NF-κB pathway activation found in NP inflammation are considered as fairly important cause of intervertebral disc(IVD)degeneration.Herein,we constructed a siSTING delivery hydrogel of aldehyde hyaluronic acid(HA-CHO)and poly(amidoamine)PAMAM/siRNA complex to intervene the abnormal STING signal for IVD degeneration treatment,where the formation of dynamic Schiff base bonds in the system(siSTING@HPgel)was able to overcome the shortcomings such as low cellular uptake,short half-life,and rapid degradation of siRNA-based strategy.PAMAM not only formed complexes with siRNA to promote siRNA transfection,but also served as dynamic crosslinker to construct hydrogel,and the injectable and self-healing hydrogel efficiently and steadily silenced STING expression in NP cells.Finally,the siSTING@HPgel significantly eased IVD inflammation and slowed IVD degeneration by prolonging STING knockdown in puncture-induced IVD degeneration rat model,revealing that STING pathway was a therapeutic target for IVD degeneration and such novel hydrogel had great potential for being applied to many other diseases for gene delivery. | Jiaxin Chen Haifeng Zhu Yutao Zhu Chenchen Zhao Shengyu Wang Yixin Zheng Ziang Xie Yang Jin Honghai Song Linjun Yang Jin Zhang Jiayong Dai Zhijun Hu Huaiyu Wang | 2022 | Bioactive Materials2022，7，3： | 2 |
| 5 | Light-induced phosphine-catalyzed asymmetric functionalization of benzylic C–H bonds显示文摘Despite rapid development in the past two decades,there are still some unsolved synthetic challenges in the field of phosphine catalysis.In this report,through photo-induced activation of ortho-alkyl aromatic ketones,we achieved highly enantioselective functionalization of substrates bearing a benzylic C–H bond.In the presence of amino acid-derived bifunctional phosphine catalysts,a range of benzylic allylation products were obtained in good yields and with excellent enantioselectivities.The strategy disclosed herein offers new insight into the activation and functionalization of pronucleophiles containing less acidic C–H bonds in the domain of phosphine catalysis and beyond. | Jiami Guo Zi-An Shen Xueting Zhou Lei Dai Yixin Lu | 2023 | Science China Chemistry2023，66，1： | 1 |
| 6 | Optimal planning of distribution substation locations and sizes-model and algorithm 显示文摘 | Dai Hongwei Yu Yixin Huang Chunhua | 1996 | Electrical Power & Energy Systems1996，18，6： | 1 |
| 7 | Optimal planning of distribution substation locations and sizes-model and algorithm 显示文摘 | Dai Hongwei Yu Yixin Huang Chunhua | 1996 | Electrical Power & Energy Systems1996，18，6： | 1 |
| 8 | Optimal planning of distribution substation location and sizes-model and algorithm 显示文摘 | Dai Hongwei Yu Yixin Huang Chunhua | 1996 | Electrical PowerandEnergySystems1996，18，6： | 1 |
| 9 | Optimal planning of distribution substation locations and sizes-model and algorithm显示文摘 | Hongwei Dai Yixin Yu Chunhua Huang | 1996 | International Journal of Electrical Power and Energy System1996，18，6： | 1 |
| 10 | Economy, environmental assessment and energy conservation for separation of isopropanol/diisopropyl ether/water multi-azeotropes via extractive distillation coupled pervaporation process显示文摘This wok proposed the extraction distillation coupled pervaporation(ED+PV) technology process using two different solvents to separate isopropanol(IPA) and diisopropyl ether(DIPE) from DIPE/IPA/H_(2)O ternary heterogeneous azeotropes in industrial wastewater from the synthesis of isopropanol in this study.Based on strict design specifications, simulation and sequential iteration methods are used for process design and optimization. Compared to the ethylene glycol(EG)-EG+H_(2)O process and the 1,3-propanediol(PDO)-IPA+H_(2)O process, the total annual cost(TAC) of the EG-IPA+H_(2)O process decreased by 20.76% and 7.86%(PDO). Compared to the EG-EG+H_(2)O process, the TAC of the PDO-IPA+H_(2)O process reduced 14%, but the global warming potential(GWP) and human toxicity of the PDO-IPA+H_(2)O process increased 11.3% and 4.07% respectively. Compared to the PDO-IPA+H_(2)O process, the EG-IPA+H_(2)O process saves 7.86%(TAC), 9.78%(GWP) and 9.85%(human toxicity). The ED+PV process with EG is superior to PDO in factors of TAC, energy consumption, human toxicity and environment. The EG-IPA+H_(2)O process changed the separation order of the products of the multi-azeotropic system, reduced the cost and energy conservation of the system, and enhanced the environmental protection evaluation of the process, is the best process through life cycle assessment for analyzing the economy, energy conservation, environmental assessment and human toxicity, designing cleaner products, controlling waste discharge, and promoting the chemical purification industry. This work provides a new process design and optimized separation ideas, will have a good guiding significance for the research and application separation of multi-azeotropic mixture with mixed solvents in organic wastewater from the cleaner chemical production, has been up to standard wastewater discharge process, and realized the development goal of carbon peak and carbon neutrality in the sustainable development of chemical clean industry. | Qinggang Xu Yasen Dai Qing Zhao Zhengrun Chen Peizhe Cui Zhaoyou Zhu Yinglong Wang Jun Gao Yixin Ma | 2023 | Chinese Journal of Chemical Engineering2023，54，2： | 1 |
| 11 | Harvesting biomechanical energy in the walking by shoe based on liquid metal magnetohydrodynamics显示文摘当走时,一个液体金属 magnetohydrodynamics 产生系统(LMMGS ) 为在鞋收集寄生力量在这份报纸被建议并且示威。不同于常规装鞋的人的力量 harvesters 那使用固体卷和齿轮机制,建议系统作为精力搬运人采用液体金属(Ga62In25Sn13 ) ,在不移动的地方,部分在 magnetohydrodynamics 发电机(MHG ) 被请求。当与 LMMGS 走时,脚或者压分别地被放在脚底的前面和尾部的二液体金属泵(LMP ) 。作为结果,在 LMP 的液体金属(LMP 我和 II ) 通过 MHG 被渗出并且流动(MHG 我和 II ) 在哪个电被生产。为比较,在所有部分除了 LMP 是一样的地方, LMMGS (LMMGS A, B 和 C ) 的三种类型被造。而且,有注射液体金属的不同体积的这些 LMMGS 的表演分别地被测试。试验性的结果表明 LMMGS 的产量电压和力量与注射液体金属的体积和 LMP 的尺寸增加。另外, 80mW 的最大的产量力量被 LMMGS C 与约 1.3% 的效率获得。给它没有副作用,轻重量,小尺寸和可靠性的优点, LMMGS 为驱动便携、可植入的 micro/nano 设备是很相配的例如便携传感器,药泵等等。 | Dan DAI Jing LIU Yixin ZHOU | 2012 | Frontiers in Energy2012，6，2： | 1 |
| 12 | Optimal planning of distribution substation locations and sizes-model and algorithm显示文摘 | Dai Hongwei Yu Yixin Huang Chunhua | 1993 | IEEE 10^st Conference on Computer Communication Control and Power Engineering1993，5，1： | 1 |
| 13 | Optimal planning of distribution substation location and sizes-model and algorithm 显示文摘 | DAI Hongwei YU Yixin HUANG Chunhua | 1996 | Electrical Power & Energy Systems1996，18，6： | 1 |
| 14 | Optimal planning of distribution substation location and sizes-model and algorithm显示文摘 | Dai Hongwei Yu Yixin Huang Chunhua | 1996 | Electrical Power and Energy Systems1996，18，6： | 1 |
| 15 | Institutions and intellectual property:the influence of insti- tutional forces on university patenting显示文摘 | YIXIN DAI DAVID POPP STUART BRETSCHNEIDER | 2005 | Journal of Policy Analysis and Management2005，24，3： | 1 |
| 16 | Optimal planning of distribution substation locations and sizes model and algorithm显示文摘 | Dai Hongwei Yu Yixin Huang Chunhua et a1 | | 0，，06： | 1 |
| 17 | Reduced smooth muscle-fibroblasts transformation potentially decreases intestinal wound healing and colitis-associated cancer in ageing mice显示文摘Cancer and impaired tissue wound healing with ageing are closely related to the quality of life of the elderly population.Given the increased incidence of cancer and the population ageing trend globally,it is very important to explore how ageing impairs tissue wound healing and spontaneous cancer.In a murine model of DSS-induced acute colitis and AOM/DSS-induced colitis-associated cancer(CAC),we found ageing significantly decreases intestinal wound healing and simultaneous CAC initiation,although ageing does not affect the incidence of AOM-induced,sporadic non-inflammatory CRC.Mechanistically,reduced fibroblasts were observed in the colitis microenvironment of ageing mice.Through conditional lineage tracing,an important source of fibroblasts potentially derived from intestinal smooth muscle cells(ISMCs)was identified orchestrating intestinal wound healing and CAC initiation in young mice.However,the number of transformed fibroblasts from ISMCs significantly decreased in ageing mice,accompanied by decreased intestinal wound healing and decreased CAC initiation.ISMCs-fibroblasts transformation in young mice and reduction of this transformation in ageing mice were also confirmed by ex-vivo intestinal muscular layer culture experiments.We further found that activation of YAP/TAZ in ISMCs is required for the transformation of ISMCs into fibroblasts.Meanwhile,the reduction of YAP/TAZ activation in ISMCs during intestinal wound healing was observed in ageing mice.Conditional knockdown of YAP/TAZ in ISMCs of young mice results in reduced fibroblasts in the colitis microenvironment,decreased intestinal wound healing and decreased CAC initiation,similar to the phenotype of ageing mice.In addition,the data from intestine samples derived from inflammatory bowel disease(IBD)patients show that activation of YAP/TAZ also occurs in ISMCs from these patients.Collectively,our work reveals an important role of the ageing stromal microenvironment in intestinal wound healing and CAC initiation.Furthermore,our work also identified a potential source of fibroblasts involved in colitis and CAC. | Yi Liu Yanhong Ji Ruiyi Jiang Chao Fang Gang Shi Lin Cheng Yinan Zuo Yixin Ye Xiaolan Su Junshu Li Huiling Wang Yuan Wang Yi Lin Lei Dai Shuang Zhang Hongxin Deng | 2023 | Signal Transduction and Targeted Therapy2023，8，9： | 0 |
| 18 | Asymmetric Dearomatization of Electron-Deficient Heteroarenes by a Phosphine-Catalyzed[3+2]Annulation with Vinylcyclopropanes显示文摘Asymmetric dearomatization reactions of various electron-deficient heteroarenes,including benzofurans,benzothiophenes,and indoles,have been described.Through a phosphine-catalyzed[3+2]annulation with vinylcyclopropanes,readily available heteroarene feedstocks undergo smooth dearomatization reactions,delivering a diverse array of valuable chiral cyclopentabenzodihydrofuran and cyclopentaindoline scaffolds in a highly diastero-and enantioselective manner.Notably,the employment of cyclopropanes in phosphine-mediated annulation for the dearomatization of electron-deficient arenes is unknown. | Xuan Dai Fuhao Zhang Lei Dai Yixin Lu | 2023 | CCS Chemistry2023，5，9： | 0 |
| 19 | Synthesis of zeolite Na-P1 from coal fly ash produced by gasification and its application as adsorbent for removal of Cr(Ⅵ) from water显示文摘The coal fly ash produced by gasification is estimated to be over 80 million ton per year in China by 2021.It has mainly been disposed as solid waste by landfill.There is lack of study focused on its utilization.In this paper,the coal fly ash produced by gasification was at first analyzed and then applied to synthesize zeolite as an adsorbent.The effects of synthesis conditions on the cation exchange capacity(CEC)of zeolite were investigated.The results from X-ray diffraction and scanning electron microscope indicated that the crystallinity of the synthesized zeolite is the most important factor to affect the CEC.When the synthesized zeolite with the highest CEC(275.5 meq/100 g)was used for the adsorption of Cr(Ⅵ) from aqueous solution,the maximum adsorption capacity for Cr(Ⅵ) was found to be 17.924 mg/g.The effects of pH,contact time and initial concentration on the adsorption of Cr(Ⅵ) were also investigated.The adsorption kinetics and isotherms can be well described by the pseudo-secondorder model and Langmuir isotherm model,respectively. | Yixin Zhang Lu Zhou Liqing Chen Yang Guo Fanhui Guo Jianjun Wu Baiqian Dai | 2021 | Frontiers of Chemical Science and Engineering2021，15，3： | 0 |
| 20 | Timing of the formation of the Baiyinnuo'er skarn Zn–Pb deposit,NE China:evidence from sulfide Rb–Sr dating显示文摘The Baiyinnuo’er deposit in northern China is located in the south section of the Great Xing’an Range,and it is the largest skarn Zn–Pb deposit in the region.Skarn and Zn–Pb orebodies mainly occur between the different units of the Permian Huanggangliang Formation,or within the contact zone between the intrusive rocks and the marble.Although Baiyinnuo’er has been well investigated previously,the timing of the Zn–Pb mineralization is still controversial,largely due to the lack of appropriate ore or alteration minerals that could be directly used for isotopic dating.In this study,we report the results of Rb–Sr isotopic analysis for sphalerite and pyrite samples from the Baiyinnuo’er orebodies,which yielded two isochron ages of 137.4±3.4 and 140.0±7.8 Ma,respectively,constraining the Zn–Pb mineralization time of the deposit as the Early Cretaceous.The data are also consistent with the age of the granitoids in the mining area,indicating a potential genetic relationship between the Early Cretaceous magmatism and mineralization.Many other intrusion-related hydrothermal deposits(including the two typical skarns,Huanggang and Haobugao)in the southern Great Xing’an Range also share similar mineralization ages(i.e.,140–130 Ma).Together,these data suggest an Early Cretaceous mineralization event in this region,and this largescale mineralization could be related to the regional tectonic regime transition from compression to extension as a result of the rollback of the subducted Paleo-Pacific plate.The initial87 Sr/86 Sr ratios of the sphalerite and pyrite samples are 0.70569 and 0.70616,respectively,implying that the ore-forming material could have a significant contribution from the mantle components.The current study shows that sulfide Rb–Sr dating could be used in deciphering the timing of skarn deposit formation. | Yixin Li Qihai Shu Xudong Niu Fan Yu Qingwen Zeng Liangmin Wei Yang Xiao Xianglin Dai | 2022 | Acta Geochimica2022，41，2： | 0 |
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