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| 1 | Concentrations and gas-particle partitioning of PCDD/Fs in the urban air of Dalian,China显示文摘PCDD/Fs in the urban air of Dalian,China were monitored with high-volume active sampler from November 2009 to October 2010.The concentration of Cl 4-8 DD/Fs ranged from 3065 to 49538 fg m-3,with an average of 10249 fg m-3.The international toxic equivalents(I-TEQ) value of that was 61.8 1182 fg m-3,with an average of 235 fg m-3,which was comparable to those in the other urban locations around the world.It was found that the Cl 4 8 DD/Fs appeared to be present mainly in the particle phase during winter,spring and autumn,while during summer which were dominantly in gas phase.The ratio of Cl 4-8 DD/Fs present in particle phase increased with the increasing level of chlorination.The concentrations of PCDFs and PCDDs decreased with the increase of chlorinated level,while the concentrations of 2,3,7,8-PCDDs congeners increased with the increase of chlorination level.The homolog profiles of the concentrations of PCDFs presented were higher than those of the PCDDs,which indicated the PCDD/Fs pollution source of the air in Dalian was characteristic for thermal source pollution.The correlation analysis of meteorological parameters with the concentrations of Cl 4-8 CDD/Fs was conducted using SPSS packages,and it was found that the ambient temperature and atmospheric pressure were important factors influence the concentration of PCDD/Fs in the air.The respiratory risk and intake dioxins of the residents around the sampling sites were studied in the paper.It was found that Junge-Pankow model was much more accurate in predicting the gas-particle partitioning behavior of PCDD/Fs homologues during winter,while the Harner-Bidleman model shows better agreement with the measured data during winter and summer. | QIN SongTao ZHU XiuHua WANG Wei CHEN JiPing NI YuWen LI XiaoXiao MU Jun Xu Qian SCHRAMM Karl-Werner | 2012 | Chinese Science Bulletin2012，57，26： | 10 |
| 2 | Experimental cancer gene therapy by multiple anti-survivin hammerhead ribozymes显示文摘为癌症改进基因治疗的功效,我们设计了指向 survivin mRNA 的暴露的区域的四撞木鲛 ribozyme 侵入人体气管粘膜的病菌(到 R4 的 R1 ) 。除了在里面 vitro 描述,由教材扩展包括了劈开的顺序特性的一颗决心,为细胞增长并且为的试金在 vivo 肿瘤,生长被用来为 ribozyme 效率得分。survivin 表示的产生抑制经由 caspase-3-dependent 小径导致了有丝分裂的大祸和房间死亡。重要地, ribozyme 侵入人体气管粘膜的病菌的管理在一个 hepato 细胞的癌异种皮移植老鼠模型禁止了肿瘤生长。R1, R3 和 R4 ribozymes 的合作表示 synergistically 压制了 survivin 并且当这联合指向 survivin 抄本的所有主要形式,生产了大多数有势力反癌症效果。带在这份报告描述的多重撞木鲛 ribozymes 的侵入人体气管粘膜的病菌对癌症提供了柔韧的基因治疗策略。 | Qi Fei Hongyu Zhang Lili Fu Xinlan Dai Baomei Gao Min Ni Chao Ge Jinjun Li Xia Ding Yuwen Ke Xuebiao Yao Jingde Zhu | 2008 | Acta Biochimica et Biophysica Sinica2008，40，6： | 10 |
| 3 | Simultaneous monitoring of PCB profiles in the urban air of Dalian,China with active and passive samplings显示文摘The concentration of polychlorinated biphenyls (PCBs) in the urban air of Dalian, China was monitored from November 2009 to October 2010 with active high-volume sampler and semipermeable membrane device (SPMD) passive sampler. The concentration of PCBs (particle + gas) ( ∑ PCBs) ranged from 18.6 to 91.0 pg/m 3 , with an average of 50.9 pg/m 3 , and the most abundant dioxin-like PCB (DL-PCBs) was PCB118. The WHO-TEQ values of DL-PCBs were 3.6-22.1 fg/m3 , with an average of 8.5 fg/m 3 , and PCB126 was the maximum contributor to ∑ TEQ. There was a much larger amount of PCBs in the gas phase than in the particulate phase. The dominant PCB components were lower and middle molecular weight PCBs. With increasing chlorination level, the concentration of the PCB congeners in the air decreased. The gas-particulate partitioning of PCBs was different for the four seasons. The gas- particulate partitioning coefficients (logK p ) vs. subcooled liquid vapor pressures (logP L 0 ) of PCBs had reasonable correlations for different sampling sites and seasons. The absorption mechanism contributed more to the gas-particulate partitioning process than adsorption. Correlation analysis of meteorological parameters with the concentration of PCBs was conducted using SPSS packages. The ambient temperature and atmospheric pressure were important factors influencing the concentration of PCBs in the air. The distribution pattern of the congeners of PCBs and the dominant contributors to DL-PCBs and TEQ in active samples and SPMDs passive samples were similar. SPMD mainly sequestrated gas phase PCBs. | Qian Xu Xiuhua Zhu Bernhard Henkelmann Karl-Werner Schramm Jiping Chen Yuwen Ni Wei Wang Gerd Pfister Jun Mu Songtao Qin Yan Li | 2013 | Journal of Environmental Sciences2013，25，1： | 8 |
| 4 | Influence of variation in the operating conditions on PCDD/F distribution in a full-scale MSW incinerator 显示文摘 | Zhang Haijun Ni Yuwen Chen Jiping | 2008 | Chemosphere2008，70，4： | 1 |
| 5 | Emissions of PCDD/Fs from municipal solid waste incinerators in China 显示文摘 | Yuwen Ni Haijun Zhang Su Fan | 2009 | Chemosphere2009，，75： | 1 |
| 6 | Emissions of PCDD/Fs from municipal solid waste incinerators in China 显示文摘 | NI Yuwen ZHANG Haijun FAN Su | 2009 | Chemosphere2009，75，9： | 1 |
| 7 | Stack gas emissions of PCDD/Fs from hospital waste incinerators in China显示文摘 | Hongcai Gao Yuwen Ni Haijun Zhang Liang Zhao Ning Zhang Xueping Zhang Qing Zhang Jiping Chen | 2009 | Chemosphere2009，，5： | 1 |
| 8 | Influ- ence of variation in the operating conditions on PC- DD/F distribution in a full-scale MSW incinerator 显示文摘 | Zhang Haijun Ni Yuwen Chen Jiping | 2008 | Chemosphere2008，70，： | 1 |
| 9 | Stack gas emissions of PCDD/Fs from hospital waste incinerators in China显示文摘 | Hongcai Gao Yuwen Ni Haijun Zhang Liang Zhao Ning Zhang Xueping Zhang Qing Zhang Jiping Chen | 2009 | Chemosphere2009，，5： | 1 |
| 10 | Study on the double transmission of ultrasonic waves through statistic rough surfaces显示文摘A model evaluating the signal loss of the double transmitted acoustic beams through random rough surfaces was established based on the Fresnel approximation and phase- screen approximation. A simple analytical solution was achieved using the exponential substi- tution approach to remove the nonlinear integral terms. The factors that affect the signal of double transmissions from random rough surfaces were analyzed. The research results demon- strated that the signal loss is not only related to the root-mean-squire height of the roughness, but also to the distance of wave traveling in the materials. The model can be very helpful for improving the reliability of NDT (Non-Destructive Testing). | CHEN Ziqiang, CHEN Ligong, NI Chunzhen, WANG Yuwen (Welding Research Institute, Shanghai Jiaotong University Shanghai 200030) | 2002 | Chinese Journal of Acoustics2002，21，2： | 1 |
| 11 | Emissions of PCDD/Fs from municipal solid waste incinerators in China显示文摘 | Yuwen Ni Haijun Zhang Su Fan | | 0，，09： | 1 |
| 12 | Stack gas emissions of PCDD/Fs from hospital waste incinerators in China显示文摘 | Gao Hongcai Ni Yuwen Zhang Haijun | | 0，，05： | 1 |
| 13 | Temperature and pH dependent morphology and FT-1R analysis of magnesium carbon-ate hydrates 显示文摘 | ZHANG Zhiping ZHENG Yajun NI Yuwen | 2006 | J Phys Chem B2006，110，12： | 1 |
| 14 | Thermal Degradation of PCDD/Fs Promoted by Alcohol Amines in Different Types of Incinerator Ashes显示文摘The low-temperature thermal treatment to degrade PCDD/Fs contained in fly ash was promoted by alcohol amines in a closed system. Three types of fly ash collected separately from municipal solid waste incinerator, medical waste incinerator and hazardous waste incinerator, were compared. Experimental design was used to investigate the homologue patterns of PCDD/Fs and distribution of the toxic congeners in fly ash from incinerator after thermal treatment promoted by alcohol amines. The effect of ethanolamine (MEA) on the hydrodechlorination reaction of polychlorinated aromatics pollutants on fly ash from solid waste incinerator was carried out, and the three ashes clearly showed different degradation potentials for PCDD/F during thermal treatment. Results from the present study indicate that (1) the concentration of alkaline species and metals strongly influenced the degradation of PCDD/F; (2) after addition of 8% MEA, the toxicity equivalent (TEQ) values of PCDD/Fs in fly ash were significantly lower than those obtained without MEA. 49%–71% of PCDD/Fs in TEQ was removed from different types of ash at 250℃ with 8% MEA; (3) the destruction and dechlorination are major mechanism for PCDD/Fs degradation. | FAN Yun ZHU Meiwen NI Yuwen CHEN Jiping CHEN Mengjun | 2013 | 矿物学报2013，33，S1： | 0 |
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