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| 1 | Adsorption separation of carbon dioxide, methane and nitrogen on monoethanol amine modified β-zeolite显示文摘A new type of composite adsorbents was synthesized by incorporating monoethanol amine (MEA) into β-zeolite. The parent and MEA- functionalized β-zeolites were characterized by X-ray diffraction (XRD), N2 adsorption, and thermogravimetric analysis (TGA). The adsorption behavior of carbon dioxide (CO2), methane (CH4), and nitrogen (N2) on these adsorbents was investigated at 303 K. The results show that the structure of zeolite was well preserved after MEA modification. In comparison with CH4 and N2, CO2 was preferentially adsorbed on the adsorbents investigated. The introduction of MEA significantly improved the selectivity of both CO2/CH4 and CO2/N2, the optimal selectivity of CO2/CH4 can reach 7.70 on 40 wt% of MEA-functionalized β-zeolite (MEA(40)-β) at 1 atm. It is worth noticing that a very high selectivity of CO2/N2 of 25.67 was obtained on MEA(40)-β. Steric effect and chemical adsorbate-adsorbent interaction were responsible for such high adsorption selectivity of CO2. The present MEA-functionalized β-zeolite adsorbents may be a good candidate for applications in flue gas separation, as well as natural gas and landfill gas purifications. | Xiaoliang Xu Xingxiang Zhao Linbing Sun Xiaoqin Liu | 2009 | Journal of Natural Gas Chemistry2009，18，2： | 11 |
| 2 | Adsorption separation of carbon dioxide,methane,and nitrogen on Hβand Na-exchangedβ-zeolite显示文摘二氧化碳的吸附等温线(公司 2), 甲烷(CH 4), 和氮(Hβ 和钠上的 N 2) 交换了 β-zeolite (Naβ) 容量的联盟者在 273 和 303 K 被测量。结果证明所有等温线具有 Brunauer 类型我和井与 Langmuir-Freundlich 相关模型。在钠离子交换以后,吸附增加的三种被吸附物质总计,当公司 2 吸附能力的增加大小比 CH 4 和 N 2 的高得多时。在 CH 4 上的公司 2 和在在钠交换以后提高的 N 2 上的公司 2 的选择。另外,吸附数据的起始的热在 Naβ 与 Na + 离子暗示了公司 2 分子的一个更强壮的相互作用。这些结果能在沸石被归因于和额外的框架阳离子的公司 2 的更大的静电的相互作用。然而, Naβ 在能被归功于到与 Naβ 的 N 2 的中等亲密关系的 N 2, 上在 CH 4 的选择显示出减少。装载的功能显示在 Naβ 的公司 2 的吸附介绍精力充沛地异构的侧面的吸附的 isosteric 热的变化。相反, CH 4 的吸附被发现实质上同类,它建议在 CH 4 和格子氧原子之间的分散相互作用,并且如此的相互作用不取决于沸石的可交换的阳离子。 | Xiaoliang Xu Xingxiang Zhao Linbing Sun Xiaoqin Liu | 2008 | Journal of Natural Gas Chemistry2008，17，4： | 11 |
| 3 | Mechanical properties of rock materials with related to mineralogical characteristics and grain size through experimental investigation: a comprehensive review显示文摘 | Wenjuan SUN Linbing WANG Yaqiong WANG | 2017 | Frontiers of Structural and Civil Engineering2017，11，3： | 5 |
| 4 | Cu-Ce bimetal ion-exchanged Y zeolites for selective adsorption of thiophenic sulfur显示文摘 | Shah Jiahui Liu Xiaoqin Sun Linbing | 2008 | Energy & Fuels2008，22，： | 1 |
| 5 | Cu Ce bimetal ion-exchanged Y zeolites for selective adsorption of thiophenic sulfur显示文摘 | Shan Jiahui Liu Xiaoqin Sun Linbing | 2008 | Energy & Fuels2008，22，6： | 1 |
| 6 | A New Image Analysis Technique for Aggregate Morphology Analysis Using Two-dimensional Fourier Transform Method显示文摘 | Sun Wenjuan Wang Linbing Erol Tutumluer | 2012 | Journal of the Transportation Research Board2012，，9： | 1 |
| 7 | Cu-Ce Bimetal ion-exchanged Y zeolites for selective adsorption of thiophenic sulfur显示文摘 | Shan Jiahui Liu Xiaoqin Sun Linbing | 2008 | Energy & Fuels2008，22，： | 1 |
| 8 | Magnetically responsive porous materials for efficient adsorption and desorption processes显示文摘Magnetically responsive porous materials possess unique properties in adsorption processes such as magneticinduced separation and heat generation in alternating magnetic fields, which greatly facilitates recycling procedures, favors long-term operation, and improves desorption rate, making conventional adsorption processes highly efficient. With increasing interest in magnetic adsorbents, great progress has been made in designing and understanding of magnetically responsive porous materials varying from monoliths to nanoscale particles used for adsorption including oil uptake, removal of hazardous substances from water, deep desulfurization of fuels, and CO2 capture in the past few years. Therefore, a review summarizing the advanced strategies of synthesizing these magnetically responsive adsorbents and the utilization of their magnetism in practical applications is highly desired. In this review, we give a comprehensive overview of this emerging field, highlighting the strategies of exquisitely incorporating magnetism to porous materials and subtly exploiting their magnetic responsiveness. Further innovations for fabricating or utilizing magnetic adsorbents are expected to be fueled. The potential opportunities and challenges are also discussed. | Peng Tan Yao Jiang Xiaoqin Liu Linbing Sun | 2019 | Chinese Journal of Chemical Engineering2019，27，6： | 1 |
| 9 | Decorating MXene with tiny ZIF-8 nanoparticles:An effective approach to construct composites for water pollutant removal显示文摘MXenes have attracted increasing research enthusiasm owing to their unique physical and chemical properties.Although MXenes exhibit exciting potential in cations adsorption due to their unique surface groups,the adsorption capacity is limited by the low specific surface area and undeveloped porosity.Our work aims at enhancing the adsorption performance of a well-known MXene,Ti3C2Tx,for methylene blue(MB)by decorating tiny ZIF-8 nanoparticles in the interlayer.After the incorporation of ZIF-8,suitable interspace in the layers resulting from the distribution of tiny ZIF-8 appears.When employing in MB,the adsorption capacity of composites can reach up to 107 mg·g^(-1) while both ZIF-8(3 mg·g^(-1))and Ti_(3)C_(2)Tx(9mg·g^(-1))show nearly no adsorption capacity.The adsorption mechanism was explored,and the good adsorption capacity is caused by the synergistic effect of ZIF-8 and Ti_(3)C_(2)Tx,for neither of them is of suitable interspace or surface groups for MB adsorption.Our work might pave the way for constructing functional materials based on the introduction of nanoparticles into layered materials for various adsorption applications. | Chen Gu Wenqiang Weng Cong Lu Peng Tan Yao Jiang Qiang Zhang Xiaoqin Liu Linbing Sun | 2022 | Chinese Journal of Chemical Engineering2022，35，2： | 1 |
| 10 | Correction To:Intranasal booster using an Omicron vaccine confers broad mucosal and systemic immunity against SARSCoV-2 variants显示文摘Correction to:Signal Transduction and Targeted Therapy http://gffzzd3cc09b8251d45dfsvc66p0wnwoon659c.ffgz.tsg.suse.edu.cn/10.1038/s41392-023-01423-6,published online 17 April 2023 After online publication of the article^(1),the authors noticed two inadvertent mistakes occurred in References that needs to be corrected.The correct text is provided as follows. | Qian Wang Chenchen Yang Li Yin Jing Sun Wei Wang Hengchun Li Zhengyuan Zhang Si Chen Bo Liu Zijian Liu Linjing Shi Xiaolin Liu Suhua Guan Chunhua Wang Linbing Qu Ying Feng Xuefeng Niu Liqiang Feng Jincun Zhao Pingchao Li Ling Chen Nanshan Zhong | 2023 | Signal Transduction and Targeted Therapy2023，8，6： | 1 |
| 11 | Evaluating carbon dioxide emissions in international trade of China显示文摘 | LinB Sun C | 2010 | Energy Policy2010，38，1： | 1 |
| 12 | Acti- vated carbon-catalyzed hydrogen transfer to α, ω- diarylalkanes 显示文摘 | Sun Linbing Zong Zhimin Kou Jiahui | 2005 | Energy & Fuels2005，19，1： | 1 |
| 13 | Fabrication of adsorbents with enhanced CuⅠ stability: Creating a superhydrophobic microenvironment through grafting octadecylamine显示文摘In atmospheric conditions, CuⅠis easily oxidized to CuⅡdue to the coexistence of moisture and oxygen.The poor oxidation inhibition of CuⅠrestricts the practical application of CuⅠ-containing materials.Herein we introduce an approach to construct a superhydrophobic microenvironment in CuⅠfunctionalized metal–organic frameworks by coordinatedly grafting organic amine compounds onto open metal sites(OMSs), which can hinder the accessibility of moisture to pores thereby enhancing the stability of CuⅠ. As a proof of concept, MIL-101(Cr) with abundant OMSs and octadecylamine(OA)with long hydrophobic alkyl groups are used as carrier and surface coating. As superhydrophobic porous materials, the resultant CuⅠM-OA exhibits improved CuⅠstability in addition to retaining high crystallinity and intact porosity while almost all CuⅠis oxidized in hydrophilic CuⅠM upon exposure in a humid atmosphere for 30 h. CuⅠM-OA owns excellent adsorption desulfurization performance(ADS) with regard to thiophene, benzothiophene, and 4,6-dimethyl dibenzothiophene. Even from hydrated fuel, the adsorption performance of CuⅠM-OA maintains well while the adsorption capacity of CuⅠM decreases to 7% after4 cycles. The remarkable moisture resistance, CuⅠstability, and high porosity make the current adsorbent CuⅠM-OA highly promising for the practical ADS process. | Zida Ma Yuxia Li Mengmeng Jin Xiaoqin Liu Linbing Sun | 2023 | Chinese Journal of Chemical Engineering2023，55，3： | 0 |
| 14 | Light-responsive adsorbentswithtunableadsorbent-adsorbate interactions forselective CO_(2) capture显示文摘Amines in porous materials have been employed as active species for the selective CO_(2) adsorption from natural gas because of their target-specific interactions.Nevertheless,it is difficult to modulate such strong interactions to reach a high efficiency in the adsorption processes.Herein,we fabricated lightresponsive adsorbents with tunable adsorbent–adsorbate interactions for CO_(2) capture.The adsorbents were synthesized by introducing primary and secondary amines into a mesoporous silica that had been grafted with azobenzene groups on the surfaces.The target-specific amine sites render the adsorbents significantly selective in the uptake of CO_(2) over CH_(4),and the azobenzene groups were used as lightresponsive switches to influence the adsorbent–adsorbate interactions.The adsorbents can freely adsorb CO_(2) when the azobenzene groups are in the trans state.Ultraviolet-light irradiation makes the azobenzene groups transform to the cis configuration,which greatly hinders amines in the uptake of CO_(2).The caused difference of adsorption capacity can reach 34.9%.The alternative irradiation by ultravioletand visible-light can lead to a recyclable regulation on adsorption performance.The changes of the electrostatic potentials of amines are responsible for the light-induced regulation on adsorption. | Peng Tan Yao Jiang Qiurong Wu Chen Gu Shichao Qi Qiang Zhang Xiaoqin Liu Linbing Sun | 2022 | Chinese Journal of Chemical Engineering2022，35，2： | 0 |
| 15 | Intranasal booster using an Omicron vaccine confers broad mucosal and systemic immunity against SARS-CoV-2 variants显示文摘The highly contagious SARS-CoV-2 Omicron subvariants severely attenuated the effectiveness of currently licensed SARS-CoV-2 vaccines based on ancestral strains administered via intramuscular injection.In this study,we generated a recombinant,replication-incompetent human adenovirus type 5,Ad5-S-Omicron,that expresses Omicron BA.1 spike.Intranasal,but not intramuscular vaccination,elicited spike-specific respiratory mucosal IgA and residential T cell immune responses,in addition to systemic neutralizing antibodies and T cell immune responses against most Omicron subvariants.We tested intranasal Ad5-S-Omicron as a heterologous booster in mice that previously received intramuscular injection of inactivated ancestral vaccine.In addition to inducing serum broadly neutralizing antibodies,there was a significant induction of respiratory mucosal IgA and neutralizing activities against Omicron subvariants BA.1,BA.2,BA.5,BA.2.75,BF.7 as well as pre-Omicron strains Wildtype,Beta,and Delta.Serum and mucosal neutralizing activities against recently emerged XBB,BQ.1,and BQ.1.1 could also be detected but were much lower.Nasal lavage fluids from intranasal vaccination contained multimeric IgA that can bind to at least 10 spike proteins,including Omicron subvariants and pre-Omicron strains,and possessed broadly neutralizing activities.Intranasal vaccination using Ad5-S-Omicron or instillation of intranasal vaccinee’s nasal lavage fluids in mouse nostrils protected mice against Omicron challenge.Taken together,intranasal Ad5-S-Omicron booster on the basis of ancestral vaccines can establish effective mucosal and systemic immunity against Omicron subvariants and multiple SARS-CoV-2 variants.This candidate vaccine warrants further development as a safe,effective,and user-friendly infection and transmission-blocking vaccine. | Qian Wang Chenchen Yang Li Yin Jing Sun Wei Wang Hengchun Li Zhengyuan Zhang Si Chen Bo Liu Zijian Liu Linjing Shi Xiaolin Liu Suhua Guan Chunhua Wang Linbing Qu Ying Feng Xuefeng Niu Liqiang Feng Jincun Zhao Pingchao Li Ling Chen Nanshan Zhong | 2023 | Signal Transduction and Targeted Therapy2023，8，5： | 0 |
| 16 | Anion-cation dual doping: An effective electronic modulation strategy of Ni2P for high-performance oxygen evolution显示文摘Developing of high-performance and low-cost electrocatalysts is of great significance to reduce the overpotential and accelerated the reaction rate of oxygen evolution in water splitting and related energy conversion applications.Herein,Fe,O-dual doped Ni2P(Fe,O-Ni2P)nanoarray is successfully synthesized on carbon cloth demonstrating enhanced electrocatalytic activity and stability for oxygen evolution reaction(OER)under alkaline media.The as-synthesized Fe,O-Ni2P nanoarray exhibits obviously improved OER performance with a low overpotential of 210 mV at 10 mA cm^-2 current density and a Tafel slope of48 mV dec^-1,as well as long-term durability.The strong coupling interaction induced changes in electronic structure lead to relatively higher oxidation state and stronger oxidation ability of the Fe,O-Ni2P nanoarray,together with the high electrochemical surface area and good conductivity contribute to the superior OER performance.This work highlights the anion-cation dual doping strategy may be an effective method for fabrication of catalysts relating to energy conversion applications. | Bo Xu Xiaodong Yang Qiang Fang Linbing Du Yan Fu Yiqiang Sun Qisheng Liu Qingquan Lin Cuncheng Li | 2020 | Journal of Energy Chemistry2020，29，9： | 0 |
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