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| 1 | Phosphogypsum stabilization of bauxite residue:Conversion of its alkaline characteristics显示文摘Reduction of the high alkalinity of bauxite residue is a key problem to solve to make it suitable for plant growth and comprehensive utilization. In this study, phosphogypsum, a waste product from the phosphate fertilizer industry, was used to drive the alkaline transformation of the bauxite residue. Under optimal water washing conditions(liquid/solid ratio of 2 mL/g, 30°C, 24 hr), the impact of quantity added, reaction time and reaction mechanism during phosphogypsum application were investigated. Phosphogypsum addition effectively lowered p H levels and reduced the soluble alkalinity by 92.2%. It was found that the concentration of soluble Na and Ca ions in the supernatant increased gradually, whilst the exchangeable Na+and Ca^(2+)in solid phase changed 112 mg/kg and 259 mg/kg, respectively. Ca^(2+)became the dominant element in the solid phase(phosphogypsum addition of 2%, liquid/solid ratio of 2 mL/g, 30°C, 12 hr). X-ray diffraction data indicated that cancrinite and hydrogarnet were the primary alkaline minerals. SEM images suggested that phosphogypsum could promote the formation of stable macroaggregates, whilst the content of Ca^(2+)increased from 5.6% to 18.2% and Na reduced from 6.8% to 2.4%. Treatment with phosphogypsum could significantly promote the transformation of alkalinity cations by neutralization, precipitation and replacement reactions.This research provided a feasible method to promote soil formation of bauxite residue by phosphogypsum amendment. | Shengguo Xue Meng Li Jun Jiang Graeme J.Millar Chuxuan Li Xiangfeng Kong | 2019 | Journal of Environmental Sciences2019，31，3： | 35 |
| 2 | Electrochemical sensor for Cd2+ and Pb2+ detection based on nano-porous pseudo carbon paste electrode显示文摘An electrochemical sensor based on self-made nano-porous pseudo carbon paste electrode(nano-PPCPE)has been successfully developed,and used to detect Cd^2+ and Pb^2+.The experimental results showed that the electrochemical performance of nanoPPCPE is evidently better than both glassy carbon electrode(GCE)and pure carbon paste electrode(CPE).Then the prepared nano-PPCPE was applied to detect Cd^2+ and Pb^2+in standard solution,the results showed that the electrodes can quantitatively detect trace Cd^2+ and Pb^2+,which has great significance in electrochemical analysis and detection.The linear ranges between the target ions concentration and the D PASV current were from 0.1-3.0 μmol/L,0.05-4.0 μmol/L for Cd^2+ and Pb^2+,respectively.And the detection limits were 0.0780 μmol/L and 0.0292 μmol/L,respectively.Moreover,the preparation of the nano-PPCPE is cheap,simple and has important practical value. | Yuan Liu Taotao Li Chuxuan Ling Zhu Chen Yan Deng Nongyue He | 2019 | Chinese Chemical Letters2019，30，12： | 3 |
| 3 | A practical method for identifying key factors in the distribution and formation of heavy metal pollution at a smelting site显示文摘Smelting activities are the main pathway for the anthropogenic release of heavy metals(HMs)into the soil-groundwater environment.It is vital to identify the factors affecting HMs pollution to better prevent and manage soil pollution.The present study conducted a comprehensive investigation of HMs in soil from a large abandoned Zn smelting site.An integrated approach was proposed to classify and quantify the factors affecting HMs pollution in the site.Besides,the quantitative relationship between hydrogeological characteristics,pollution transmission pathways,smelting activities and HMs pollutionwas established.Results showed that the soils were highly contaminated by HMs with a pollution index trend of As>Zn>Cd>Pb>Hg.In identifying the pollution hotspots,we conclude that the pollution hotspots of Pb,As,Cd,and Hg present a concentrated distribution pattern.Geo-detector method results showed that the dominant driving factors for HMs distribution and accumulation were the potential pollution source and soil permeability.Additionally,the main drivers are variable for different HMs,and the interaction among factors also enhanced soil HMs contamination.Our analysis illustrates how the confounding influences from complex environmental factors can be distilled to identify key factors in pollution formation to guide future remediation strategies. | Jiaqing Zeng Wenshun Ke Min Deng Jingqiang Tan Chuxuan Li Yizhi Cheng Shengguo Xue | 2023 | Journal of Environmental Sciences2023，，5： | 3 |
| 4 | Optical orbital angular momentum multiplexing communication via inversely-designed multiphase plane light conversion显示文摘Multiplexing and demultiplexing of optical orbital angular momentum(OAM)are critical operations in modedivision multiplexing communications.Traditional Dammann gratings,spiral phase planes,and optical geometric transformations are regarded as convenient methods for OAM mode(de)multiplexing.However,crosstalk between the different modes and the difficulty of mode multiplexing greatly limit their application to modedivision multiplexing communications.Here,using a set of inversely-designed phase planes,we demonstrate an OAM(de)multiplexer based on multiphase plane light conversion that can enable perfect OAM multiplexing communication.The sorted patterns are Gaussian-like and can be coupled easily into single-mode fiber arrays.Inputs from the fiber array are turned into coaxial OAM modes after the phase planes.OAM mode crosstalk generated by the multiplexer is less than-20 d B,with insertion loss of less than 2.6 d B.OAM modes are sorted by the demultiplexer with mode crosstalk below-10 d B,and the sorting results are coupled to the fiber array.OAM modes carrying 10 Gbit/s on–off keying signals were transmitted in a 5 km few-mode fiber.The measured bit-error-rate curves have power penalties of less than 10 d B.The proposed configuration is highly efficient and convenient and will be beneficial for potential applications in quantum information,information processing,and optical communications. | JUNCHENG FANG JINPEI LI ARU KONG YOUPENG XIE CHUXUAN LIN ZHENWEI XIE TING LEI XIAOCONG YUAN | 2022 | Photonics Research2022，10，9： | 3 |
| 5 | Mechanical activation of spike fosters SARS-CoV-2 viral infection显示文摘The outbreak of SARS-CoV-2(SARS2)has caused a global COVID-19 pandemic.The spike protein of SARS2(SARS2-S)recognizes host receptors,including ACE2,to initiate viral entry in a complex biomechanical environment.Here,we reveal that tensile force,generated by bending of the host cell membrane,strengthens spike recognition of ACE2 and accelerates the detachment of spike’s S1 subunit from the S2 subunit to rapidly prime the viral fusion machinery.Mechanistically,such mechano-activation is fulfilled by force-induced opening and rotation of spike’s receptor-binding domain to prolong the bond lifetime of spike/ACE2 binding,up to 4 times longer than that of SARS-S binding with ACE2 under 10 pN force application,and subsequently by force-accelerated S1/S2 detachment which is up to~103 times faster than that in the no-force condition.Interestingly,the SARS2-S D614G mutant,a more infectious variant,shows 3-time stronger force-dependent ACE2 binding and 35-time faster force-induced S1/S2 detachment.We also reveal that an anti-S1/S2 non-RBD-blocking antibody that was derived from convalescent COVID-19 patients with potent neutralizing capability can reduce S1/S2 detachment by 3×106 times under force.Our study sheds light on the mechano-chemistry of spike activation and on developing a non-RBD-blocking but S1/S2-locking therapeutic strategy to prevent SARS2 invasion. | Wei Hu Yong Zhang Panyu Fei Tongtong Zhang Danmei Yao Yufei Gao Jia Liu Hui Chen Qiao Lu Tenny Mudianto Xinrui Zhang Chuxuan Xiao Yang Ye Qiming Sun Jing Zhang Qi Xie Pei-Hui Wang Jun Wang Zhenhai Li Jizhong Lou Wei Chen | 2021 | Cell Research2021，31，10： | 2 |
| 6 | Alkalinity neutralization and structure upgrade of bauxite residue waste via synergistic pyrolysis with biomass显示文摘Bauxite residues,a large volume solid waste,are in urgent need of effective disposal and management.Especially,strategies to alleviate the high alkalinity of bauxite residue remain a big challenge.Here,we developed a synergistic pyrolysis to neutralize the alkalinity of bauxite residue and upgrade the structure of biomass simultaneously.By cooperating the catalytic feature from bauxite residue,rice straw,a cellulose-enriched biomass,could prefer to produce acidic components under a hypothermal pyrolysis temperature(below 250℃)and partial oxygen-contained atmosphere as evidenced by the synchronous TGA-FTIR analysis.In return,these in-situ produced acidic components neutralized the bauxite residue profoundly(pH decreased from 11.5 to 7.2)to obtain a neutral product with long-term water leaching stability.Also,a higher pyrolysis temperature led to neutral biochar-based products with well-defined carbonization characteristics.Thus,the biomass-driven pyrolysis strategy provides a potential to dispose the alkalinity issue of bauxite residue and further opportunities for the sustainable reuse and continuing management of bauxite residue. | Chuxuan Li Lu Tang Jun Jiang Feng Zhu Jingju Zhou Shengguo Xue | 2020 | Journal of Environmental Sciences2020，32，7： | 1 |
| 7 | Epidermal radio frequency electronics for wireless power transfer显示文摘Epidermal electronic systems feature physical properties that approximate those of the skin,to enable intimate,long-lived skin interfaces for physiological measurements,human–machine interfaces and other applications that cannot be addressed by wearable hardware that is commercially available today.A primary challenge is power supply;the physical bulk,large mass and high mechanical modulus associated with conventional battery technologies can hinder efforts to achieve epidermal characteristics,and near-field power transfer schemes offer only a limited operating distance.Here we introduce an epidermal,farfield radio frequency(RF)power harvester built using a modularized collection of ultrathin antennas,rectifiers and voltage doublers.These components,separately fabricated and tested,can be integrated together via methods involving soft contact lamination.Systematic studies of the individual components and the overall performance in various dielectric environments highlight the key operational features of these systems and strategies for their optimization.The results suggest robust capabilities for battery-free RF power,with relevance to many emerging epidermal technologies. | Xian Huang Yuhao Liu Gil Woo Kong Jung Hun Seo Yinji Ma Kyung-In Jang Jonathan A.Fan Shimin Mao Qiwen Chen Daizhen Li Hank Liu Chuxuan Wang Dwipayan Patnaik Limei Tian Giovanni A.Salvatore Xue Feng Zhenqiang Ma Yonggang Huang John A.Rogers | 2016 | Microsystems & Nanoengineering2016，2，1： | 1 |
| 8 | Accelerated alkalinity regulation and long-term dry-wet aging durability for bauxite residue remediated with biomass pyrolysis显示文摘Biomass fermentation provides a potential route toward the ecological disposal for the bauxite residue(BR)with high alkalinity issues.However,how to accelerate the remediation of the alkaline problem with a long-term durability is still a big challenge.Herein,we investigated the acceleration of the decomposition of straw toward organic acid species via a pyrolysis strategy as well as the pH stability during long-term dry-wet aging for the treated BR.The pH of pyrolytic BR at 300℃ is stabilized at around 8.90 after 70 days’dry-wet aging.During the aging,the main Ca-contained alkaline minerals of calcite and cancrinite are dissolved and the content of exchangeable Na+is reduced.This pyrolysis process can decompose straw quickly and produce more organic matters that are easily degraded to fulvic and humic acid as evidenced by 3D fluorescence spectrum analysis.Compared to the fermentation with straw under natural conditions,the alkalinity regulation of BR after pyrolysis is featured with shorter period and lower pH as well as long-term pH stability.Therefore,the synergistic pyrolysis of BR with straw provides an alternative method to address the alkaline issues,which is conducive to promoting the soil formation of BR. | Zhexiang He Jingju Zhou Jianwei Tang Chuxuan Li Jun Jiang Wei Chen Feng Zhu Shengguo Xue | 2022 | Journal of Environmental Sciences2022，34，1： | 0 |
| 9 | Insights into the dwarfing mechanism of pear(Pyrus betulaefolia) based on anatomical and structural analysis using X-ray scanning显示文摘The lack of a suitable rootstock to control scion growth has limited the development of high-density plantations in pear production, which is partly attributed to poor understanding of the dwarfing mechanism. In the present study, the rootstock of the dwarf-type pear (Pyrus betulaefolia)PY-9’ was identified and used as the material for anatomical analysis.PY-9’ grew to half the tree height of the normal cultivar Zhengdu’, along with fewer internodes and shorter length. Significant differences in growth rate betweenPY-9’ andZhengdu’ were detected at approximately 30 days after full bloom, which corresponded with the time of the greatest difference in water potential between the dwarf and normal cultivar.PY-9’ showed a higher photosynthetic rate thanZhengdu’. Anatomical analysis showed thatPY-9’ had higher area ratios of both phloem and xylem and more developed vascular tissues thanZhengdu’. The three-dimensional reconstructed skeleton of the xylem from X-ray computed tomography scanning revealed greater intervessel connectivity inZhengdu’ than inPY-9’, which could contribute to the more vigorous growth ofZhengdu’. This study thus provides the first comparison of the microstructural properties of xylem elements between a dwarfing-type and vigorous-type pear rootstock, providing new insights into the dwarfing mechanism in pear and facilitating breeding of dwarf pear rootstocks to increase crop productivity. | Lili Dong Chuxuan Yang Jing Wang Jingjing Li Mei Zhao Dingli Li Zhiyun Qiu Chunhui Ma Zhenhua Cui | 2024 | Horticultural Plant Journal2024，10，2： | 0 |
| 10 | A simple visual method for DNA detection based on the formation of gold nanoparticles显示文摘A simple visual method for DNA detection during the formation of gold nanoparticles(AuNPs) was developed based on different electrostatic properties of single strand DNA(ssDNA) and double strand DNA(dsDNA).Since the ssDNA is easy to bind to AuNPs due to its exposed bases which could prevent saltinduced aggregation of AuNPs.The dsDNA always present negative charge because its negatively charged phosphate backbone is exposed.In this case,the dsDNA could disturb the adsorption between dsDNA and AuNPs and result in non-aggregation of AuNPs.After hybridization,chloroauric acid and ascorbic acid were added to the mixture solution,and the solution changed to red immediately and turned to purple in10 min in the present of target DNA.TEM results confirmed that the change of color stemed from aggregation of AuNPs.In order to obtain accurate results by naked eye,the DNA detection assay should be conducted under pH 7.0. | Yuan Liu Taotao Li Chuxuan Ling Zunliang Wang Lian Jin Yongxiang Zhao Zhu Chen Song Li Yan Deng Nongyue He | 2019 | Chinese Chemical Letters2019，30，12： | 0 |
| 11 | RADepthNet:Reflectance-aware monocular depth estimation显示文摘Background Monocular depth estimation aims to predict a dense depth map from a single RGB image,and has important applications in 3D reconstruction,automatic driving,and augmented reality.However,existing methods directly feed the original RGB image into the model to extract depth features without avoiding the interference of depth-irrelevant information on depth-estimation accuracy,which leads to inferior performance.Methods To remove the influence of depth-irrelevant information and improve the depth-prediction accuracy,we propose RADepthNet,a novel reflectance-guided network that fuses boundary features.Specifically,our method predicts depth maps using the following three steps:(1)Intrinsic Image Decomposition.We propose a reflectance extraction module consisting of an encoder-decoder structure to extract the depth-related reflectance.Through an ablation study,we demonstrate that the module can reduce the influence of illumination on depth estimation.(2)Boundary Detection.A boundary extraction module,consisting of an encoder,refinement block,and upsample block,was proposed to better predict the depth at object boundaries utilizing gradient constraints.(3)Depth Prediction Module.We use an encoder different from(2)to obtain depth features from the reflectance map and fuse boundary features to predict depth.In addition,we proposed FIFADataset,a depth-estimation dataset applied in soccer scenarios.Results Extensive experiments on a public dataset and our proposed FIFADataset show that our method achieves state-of-the-art performance. | Chuxuan LI Ran YI Saba Ghazanfar ALI Lizhuang MA Enhua WU Jihong WANG Lijuan MAO Bin SHENG | 2022 | Virtual Reality & Intelligent Hardware2022，4，5： | 0 |
| 12 | Novel biomonitoring method for determining five classes of legacy and alternative flame retardants in human serum samples显示文摘Flame retardants(FRs)are ubiquitous in environment and biota and may pose harm to human health.In recent years,concern regarding legacy and alternative FRs has been intensified due to their widespread production and increasing contamination in environmental and human matrices.In this study,we developed and validated a novel analytical method for simultaneous determination of legacy and alternative FRs,including polychlorinated naphthalenes(PCNs),short-and middle-chain chlorinated paraffins(SCCPs and MCCPs),novel brominated flame retardants(NBFRs),and organophosphate esters(OPEs)in human serum.Serum samples were prepared by liquid-liquid extraction using ethyl acetate,and purified with Oasis®HLB cartridge and Florisil–silica gel columns.Instrumental analyses were carried out using gas chromatography-triple quadrupole mass spectrometry,highresolution gas chromatography coupled with high-resolution mass spectrometry,and gas chromatography coupled with quadrupole time-of-flight mass spectrometry,respectively.The proposed method was validated for linearity,sensitivity,precision,accuracy,and matrix effects.Method detection limits for NBFRs,OPEs,PCNs,SCCPs,and MCCPs were 4.6×10^(–4)–8.6×10^(–2),4.3×10^(–3)–1.3,1.1×10^(–5)–1.0×10^(–4),1.5,and 9.0×10–1 ng/mL,respectively.Matrix spike recoveries ranged from 73%–122%,71%–124%,75%–129%,92%–126%,and 94%–126%for NBFRs,OPEs,PCNs,SCCPs,and MCCPs,respectively.The analytical method was applied for detection of real human serum.CPs were the dominant FRs in serum,indicating CPs were widely presented in human serum and should be pay more attention for their health risk. | Xiaolin Guan Gaoxin Zhang Lingling Meng Mei Liu Liyuan Zhang Chuxuan Zhao Yingming Li Qinghua Zhang Guibin Jiang | 2023 | Journal of Environmental Sciences2023，，9： | 0 |
| 13 | Migration and distribution characteristics of soil heavy metal(loid)s at a lead smelting site显示文摘Heavy metal(loid)s contamination is a constant issue at smelting sites.It is essential to investigate the spatial distribution and migration characteristics of heavy metal(loid)s in the soil for environmental management and remediation strategies of non-ferrous smelting sites.In this study,203 soil samples from 57 sites were collected in a typical lead smelting site.The findings demonstrated that there were significant Pb,Zn,Cd,and As contamination in soil samples.The spatial distribution of heavy metal(loid)s showed strong spatial heterogeneity,the contaminated soil areas of Pb,As,Cd,and Zn were 99.5%,98.9%,85.3%,and 72.4%,respectively.Pb,Cd,and As contamination of the soil reached a depth of 5 m,which migrated from the surface to deep soil layers.The leaching contents of Zn,Pb,and As decreased obviously in 3-4 m soil layer,but the leaching content of Cd was still high,which indicated the high migration of Cd.With the increase of depth,the proportion of acid soluble fraction of heavy metal(loid)s decreased,and the residual fraction increased.The acid soluble fraction of Cd accounted for a higher proportion,and As mainly existed in reducible and residual fractions in soil.According to the calculation of the migration factor,the migration of heavy metal(loid)s in soils were ordered as Cd>Zn>Pb>As.The outcomes are advantageous for risk reduction and site remediation for non-ferrous metal smelting sites. | Chuxuan Li Mu Li Jiaqing Zeng Shanxin Yuan Xinghua Luo Chuan Wu Shengguo Xue | 2024 | Journal of Environmental Sciences2024，，1： | 0 |
| 14 | Author Correction: Mechanical activation of spike fosters SARS- CoV-2 infection显示文摘 | Wei Hu Yong Zhang Panyu Fei Tongtong Zhang Danmei Yao Yufei Gao Jia Liu Hui Chen Qiao Lu Tenny Mudianto Xinrui Zhang Chuxuan Xiao Yang Ye Qiming Sun Jing Zhang Qi Xie Pei-Hui Wang Jun Wang Zhenhai Li Jizhong Lou Wei Chen | 2021 | Cell Research2021，31，11： | 0 |
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